Resonance enhancement of two-photon absorption in porphyrins

被引：161
|
作者：
Drobizhev, M
Karotki, A
Kruk, M
Rebane, A [1 ]
机构：
[1] Montana State Univ, Dept Phys, Bozeman, MT 59717 USA
[2] PN Lebedev Phys Inst, Moscow 11991, Russia
[3] Natl Acad Sci, Inst Mol & Atom Phys, Minsk, BELARUS
来源：
CHEMICAL PHYSICS LETTERS | 2002年 / 355卷 / 1-2期
关键词：
D O I：
10.1016/S0009-2614(02)00206-3
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Two-photon absorption spectra in absolute cross-section values are presented for a number of octaethyl-, tetraphenyl-. and tetrabenzo-substituted porphyrins. In excitation spectral region of 710-810 nm, the two-photon absorption efficiency is resonantly enhanced due to nearby Q(0-0) one-photon transition. The cross-section value calculated directly from the ground- and excited-state absorption parameters in a single intermediate level approximation, agrees well with that measured in experiment. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码：175 / 182
页数：8
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