Recovery of time evolving fluorescence spectra via sum-frequency cross-correlation frequency resolved optical gating

被引：0
|
作者：
Langdon, BT [1 ]
Levinger, NE [1 ]
机构：
[1] Colorado State Univ, Dept Chem, Ft Collins, CO 80523 USA
来源：
APPLIED PHYSICS LETTERS | 2005年 / 87卷 / 23期
基金：
美国国家科学基金会;
关键词：
D O I：
10.1063/1.2138366
中图分类号：
O59 [应用物理学];
学科分类号：
摘要：
Sum-frequency conversion of sample emission with short light pulses has been used for time-resolved fluorescence of chromophores in solution. In contrast to traditional fluorescence upconversion techniques where the time resolved fluorescence signal is approximated from 10 to 15 different sum-frequency gated decays distributed across the fluorescence spectrum, sum-frequency cross-correlation frequency resolved optical gating offers the opportunity to determine the electric field of the sample fluorescence as a function of time. Dynamic quantities associated with changes in the sample emission, such as solvent relaxation, can then be obtained directly from the electric field without assumption of a particular spectral line shape. (c) 2005 American Institute of Physics.
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页码：1 / 3
页数：3
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