On the Green-Kubo relationship for the liquid-solid friction coefficient

被引:83
|
作者
Bocquet, Lyderic [1 ]
Barrat, Jean-Louis [2 ]
机构
[1] Univ Lyon 1, CNRS, UMR 5306, Inst Lumiere Mat, F-69622 Villeurbanne, France
[2] Univ Grenoble 1, CNRS, UMR 5588, LiPhy, F-38402 Grenoble, France
来源
JOURNAL OF CHEMICAL PHYSICS | 2013年 / 139卷 / 04期
关键词
BOUNDARY-CONDITIONS; TRANSPORT; FLOW;
D O I
10.1063/1.4816006
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
In this paper, we propose a new derivation for the Green-Kubo relationship for the liquid-solid friction coefficient characterizing hydrodynamic slippage at a wall. It is based on a general Langevin approach for the fluctuating wall velocity involving a non-Markovian memory kernel with vanishing time integral. The calculation highlights some subtleties of the wall-liquid dynamics leading to superdiffusive motion of the fluctuating wall position. (C) 2013 AIP Publishing LLC.
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页数:4
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