Catalytic conversion wood syngas to synthetic aviation turbine fuels over a multifunctional catalyst

被引：56

作者：

Yan, Qiangu ^{[1
]}

Yu, Fei ^{[1
]}

Liu, Jian ^{[2
]}

Street, Jason ^{[1
]}

Gao, Jinsen ^{[2
]}

Cai, Zhiyong ^{[3
]}

Zhang, Jilei ^{[4
]}

机构：

[1] Mississippi State Univ, Dept Agr & Biol Engn, Mississippi State, MS 39762 USA

[2] China Univ Petr, State Key Lab Heavy Oil, Beijing 102249, Peoples R China

[3] US Forest Serv, USDA, Forest Prod Lab, Madison, WI USA

[4] Mississippi State Univ, Dept Forest Prod, Mississippi State, MS 39762 USA

来源：

BIORESOURCE TECHNOLOGY | 2013年 / 127卷

关键词：

Wood syngas; Synthetic aviation turbine fuels (SATFs); Gasification; Syngas cleaning; Multi-functional catalyst; FISCHER-TROPSCH SYNTHESIS; DIESEL PRODUCTION; HIGHER ALCOHOLS; SYNTHESIS GAS; ISOMERIZATION; BIOMASS; IRON;

D O I：

10.1016/j.biortech.2012.09.069

中图分类号：

S2 [农业工程];

学科分类号：

0828 ;

摘要：

A continuous process involving gasification, syngas cleaning, and Fischer-Tropsch (FT) synthesis was developed to efficiently produce synthetic aviation turbine fuels (SATFs). Oak-tree wood chips were first gasified to syngas over a commercial pilot plant downdraft gasifier. The raw wood syngas contains about 47% N-2, 21% CO, 18% H-2, 12% CO2 2% CH4 and trace amounts of impurities. A purification reaction system was designed to remove the impurities in the syngas such as moisture. oxygen, sulfur, ammonia, and tar. The purified syngas meets the requirements for catalytic conversion to liquid fuels. A multi-functional catalyst was developed and tested for the catalytic conversion of wood syngas to SATFs. It was demonstrated that liquid fuels similar to commercial aviation turbine fuels (Jet A) was successfully synthesized from bio-syngas. (C) 2012 Elsevier Ltd. All rights reserved.

引用

页码：281 / 290

页数：10

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