Two-photon absorption resonance effects in the third-order responses of transparent liquids

被引：9
|
作者：
Ziegler, LD
Jordanides, XJ
机构：
[1] Boston Univ, Dept Chem, Boston, MA 02215 USA
[2] Univ Calif Berkeley, Dept Chem, Berkeley, CA 94720 USA
来源：
CHEMICAL PHYSICS LETTERS | 2002年 / 352卷 / 3-4期
基金：
美国国家科学基金会;
关键词：
D O I：
10.1016/S0009-2614(01)01444-0
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Two-photon absorption (TPA) resonance effects on the ultrafast pump-probe and transient grating (TG) responses of some transparent liquids excited with 400 nm pulses are demonstrated. The contribution of TPA and ground state Raman responses are separated in a TG experiment when the third-order polarization signal is viewed in the appropriate phase-matched direction as shown for the homodyne, TG response of CS2. The pump-probe dichroic responses of liquids with (CS2 and CH3I) and without (H2O, CCl4, and CH3OH) TPA resonances at 200 nm are compared. These results are discussed in the context of a perturbative third-order polarization treatment of TPA. (C) 2002 Elsevier Science B.V. All rights reserved.
引用
收藏
页码：270 / 280
页数：11
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