Oxygen Reduction Reaction Enhancement of PdCo/C Electrocatalysts Driven by Oxidation Treatment

被引：0
|
作者：
Wei, Yu-Chen [1 ]
Liu, Chen-Wei [1 ]
Wang, Kuan-Wen [1 ]
机构：
[1] Natl Cent Univ, Inst Mat Sci & Engn, Taoyuan 320, Taiwan
来源：
CLEAN TECHNOLOGY 2011: BIOENERGY, RENEWABLES, STORAGE, GRID, WASTE AND SUSTAINABILITY | 2011年
关键词：
PdCo/C; oxidation treatment; degree of surface oxidation (DSO); oxygen reduction reaction (ORR); PdO; METHANOL FUEL-CELLS; ALLOY ELECTROCATALYSTS; CATALYSTS; PD; CARBON; SIZE; ELECTRODECOMPOSITION; ELECTROREDUCTION; NANOPARTICLES; HYDROGEN;
D O I：
暂无
中图分类号：
X [环境科学、安全科学];
学科分类号：
08 ; 0830 ;
摘要：
The effect of oxidation treatment induced progressive enhancement on oxygen reduction reaction (ORR) activities of PdCo/C catalysts is studied. Based on the XPS characterization, a new term, degree of surface oxidation (DSO), is proposed to illustrate their relationship between ORR activity and surface oxidation extent. It can be obviously found the optimal temperature for the promotion of ORR activity on various oxidized samples is 520 K. The improved ORR activity is ascribed to the formation of surface PdO species with 100 % DSO value.
引用
收藏
页码：395 / 398
页数：4
相关论文
共 50 条
  • [1] Oxygen Reduction Reaction Enhancement of PdCo/C Electrocatalysts Driven by Oxidation Treatment
    Wei, Yu-Chen
    Liu, Chen-Wei
    Wang, Kuan-Wen
    NANOTECHNOLOGY 2011: ADVANCED MATERIALS, CNTS, PARTICLES, FILMS AND COMPOSITES, NSTI-NANOTECH 2011, VOL 1, 2011, : 662 - 665
  • [2] Improvement of oxygen reduction reaction and methanol tolerance characteristics for PdCo electrocatalysts by Au alloying and CO treatment
    Wei, Yu-Chen
    Liu, Chen-Wei
    Wang, Kuan-Wen
    CHEMICAL COMMUNICATIONS, 2011, 47 (43) : 11927 - 11929
  • [3] Phase change of bimetallic PdCo electrocatalysts caused by different heat-treatment temperatures: Effect on oxygen reduction reaction activity
    Kim, Dae-Suk
    Kim, Jun-Hyuk
    Jeong, Il-Kyoung
    Choi, Jong Kwon
    Kim, Yong-Tae
    JOURNAL OF CATALYSIS, 2012, 290 : 65 - 78
  • [4] Pd–Zn/C bimetallic electrocatalysts for oxygen reduction reaction
    Georgios Bampos
    Dimitris I. Kondarides
    Symeon Bebelis
    Journal of Applied Electrochemistry, 2018, 48 : 675 - 689
  • [5] Pd–Zn/C bimetallic electrocatalysts for oxygen reduction reaction
    Bebelis, Symeon (simeon@chemeng.upatras.gr), 1600, Springer Science and Business Media B.V. (48):
  • [6] Ultrasound-Driven enhancement of Pt/C catalyst stability in oxygen reduction reaction
    Lee, Hyunjoon
    Park, Eunbi
    Lee, Eunjik
    Lim, Iksung
    Yang, Tae-Hyun
    Park, Gu-Gon
    ULTRASONICS SONOCHEMISTRY, 2024, 102
  • [7] Ultrathin PdCu Nanosheet as Bifunctional Electrocatalysts for Formate Oxidation Reaction and Oxygen Reduction Reaction
    Liu, Zhipeng
    Xue, Jinling
    Li, Yinshi
    SMALL METHODS, 2023, 7 (07)
  • [8] Molecular electrocatalysts for the oxygen reduction reaction
    Dey, Subal
    Mondal, Biswajit
    Chatterjee, Sudipta
    Rana, Atanu
    Amanullah, S. K.
    Dey, Abhishek
    NATURE REVIEWS CHEMISTRY, 2017, 1 (12)
  • [9] Molecular electrocatalysts for the oxygen reduction reaction
    Subal Dey
    Biswajit Mondal
    Sudipta Chatterjee
    Atanu Rana
    Sk Amanullah
    Abhishek Dey
    Nature Reviews Chemistry, 1
  • [10] Methanol-Tolerant Heterogeneous PdCo@PdPt/C Electrocatalyst for the Oxygen Reduction Reaction
    Yang, J.
    Cheng, C. H.
    Zhou, W.
    Lee, J. Y.
    Liu, Z.
    FUEL CELLS, 2010, 10 (06) : 907 - 913
12345