Atomically dispersed catalysts for hydrogen/oxygen evolution reactions and overall water splitting

被引：78
|
作者：
Zhang, Qiaoqiao [1 ]
Guan, Jingqi [1 ]
机构：
[1] Jilin Univ, Coll Chem, Key Lab Surface & Interface Chem Jilin Prov, Changchun 130021, Peoples R China
来源：
JOURNAL OF POWER SOURCES | 2020年 / 471卷
关键词：
Single-atom catalyst; Electrocatalysis; Hydrogen evolution; Oxygen evolution; Overall water splitting; SINGLE-ATOM CATALYSTS; OXYGEN REDUCTION REACTION; TRANSMISSION ELECTRON-MICROSCOPY; METAL-ORGANIC FRAMEWORK; RAY-ABSORPTION SPECTROSCOPY; NITROGEN-DOPED GRAPHENE; IN-SITU; ACTIVE-SITES; PLATINUM ATOMS; POROUS CARBON;
D O I：
10.1016/j.jpowsour.2020.228446
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Recent advancement of single-atom catalysts (SACs) in electrochemical water splitting is systematically reviewed. This review focuses on various SACs including Mn, Fe, Co, Ni, Mo, Pd, Ru, Rh, Ir, and Pt with single-metal or dual-metal sites for hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and overall water splitting. The primary synthesis methods and advanced characterization techniques of SACs are documented. The geometric and electronic configurations of active sites and structure-property relationships in hydrogen and oxygen electrode reactions are highlighted. The research perspectives and challenges on the future development of SACs are provided.
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页数：19
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