Enhanced Two-Photon Absorption of Organic Chromophores: Theoretical and Experimental Assessments

被引：487

作者：

Terenziani, Francesca ^{[4
,5
]}

Katan, Claudine ^{[1
]}

Badaeva, Ekaterina ^{[6
]}

Tretiak, Sergei ^{[2
,3
]}

Blanchard-Desce, Mireille ^{[1
]}

机构：

[1] Univ Rennes 1, CNRS, F-35042 Rennes, France

[2] Los Alamos Natl Lab, Ctr Nonlinear Studies, Div Theoret, Los Alamos, NM 87545 USA

[3] Los Alamos Natl Lab, Ctr Integrated Nanotechnol, Los Alamos, NM 87545 USA

[4] Univ Parma, Dipartimento Chim GIAF, I-43100 Parma, Italy

[5] INSTM UdR Parma, I-43100 Parma, Italy

[6] Univ Washington, Dept Chem, Seattle, WA 98195 USA

来源：

ADVANCED MATERIALS | 2008年 / 20卷 / 24期

关键词：

D O I：

10.1002/adma.200800402

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Functional organic materials with enhanced two-photon absorption lead to new technologies in the fields of chemistry, biology, and photonics. In this article we review experimental and theoretical methodologies allowing detailed investigation and analysis of two-photon absorption properties of organic chromophores. This includes femtosecond two-photon excited fluorescence experimental setups and quantum-chemical methodologies based on time-dependent density functional theory. We thoroughly analyze physical phenomena and trends leading to large two-photon absorption responses of a few series of model chromophores focusing on the effects of symmetric and asymmetric donor/acceptor substitution and branching.

引用

页码：4641 / 4678

页数：38

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