Hydrogen-rich gas production by steam gasification of municipal solid waste (MSW) using NiO supported on modified dolomite

被引:136
|
作者
Wang, Jingbo [1 ]
Cheng, Gong [1 ]
You, Yanli [1 ]
Xiao, Bo [1 ]
Liu, Shiming [1 ]
He, Piwen [1 ]
Guo, Dabin [1 ]
Guo, Xianjun [2 ]
Zhang, Guijuan [1 ]
机构
[1] Huazhong Univ Sci & Technol, Sch Environm Sci & Engn, Wuhan 430074, Hubei, Peoples R China
[2] Yantai Univ, Sch Environm & Mat Engn, Yantai 264005, Peoples R China
关键词
Hydrogen-rich gas; Municipal solid waste (MSW); Gasification; NiO on modified dolomite catalysts; BIOMASS GASIFICATION; PYROLYSIS-GASIFICATION; TAR GASIFICATION; NICKEL-CATALYSTS; FLUIDIZED-BED; TEMPERATURE; RESISTANCE; MIXTURES; REMOVAL; COKING;
D O I
10.1016/j.ijhydene.2012.01.070
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
NiO on modified dolomite (NiO/MD) catalysts were developed for hydrogen-rich gas production from steam gasification of municipal solid waste (MSW). The catalysts were prepared through deposition-precipitation method and characterized by various characterization methods. The activity of NiO/MD on the steam gasification of MSW was investigated in a lab-scale fixed bed. The results indicated that the catalysts could significantly eliminate the tar in the gas production and increase the hydrogen yield. In addition, higher temperature contributed to higher hydrogen production and gas yield, meanwhile, the optimal ratio of steam to MSW (S/M) was found to be 1.23. In the experimental conditions, the NiO/MD catalysts showed a good performance over a long lifetime test. Copyright (C) 2012, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:6503 / 6510
页数:8
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