In-Operando Impedance Spectroscopy and Ultrasonic Measurements during High-Temperature Abuse Experiments on Lithium-Ion Batteries

被引：34
|
作者：
Zappen, Hendrik [1 ,2 ,3 ]
Fuchs, Georg [1 ,2 ,3 ]
Gitis, Alexander [1 ,2 ,3 ]
Sauer, Dirk Uwe [1 ,2 ,4 ,5 ]
机构：
[1] Rhein Westfal TH Aachen, Inst Power Elect & Elect Drives ISEA, Electrochem Energy Convers & Storage Syst Grp, Jaegerstr 17-19, D-52066 Aachen, Germany
[2] Forschungszentrum Julich, JARA Energy, Julich Aachen Res Alliance, D-52425 Julich, Germany
[3] Safion GmbH, Huttenstr 7, D-52068 Aachen, Germany
[4] Rhein Westfal TH Aachen, Inst Power Generat & Storage Syst PGS, EON ERC, Mathieustr 10, D-52074 Aachen, Germany
[5] Forschungszentrum Julich, Helmholtz Inst Munster HI MS, IEK 12, D-52425 Julich, Germany
来源：
BATTERIES-BASEL | 2020年 / 6卷 / 02期
关键词：
EIS; electrochemical impedance spectroscopy; lithium-ion batteries; characterization; diagnostics; abuse test; high temperature; degradation; safety; ultrasonics; ultrasound; strain; gassing; gas evolution; THERMAL-STABILITY; CATHODE MATERIALS; ELECTROLYTES; BREAKDOWN; SPECTRA; CHARGE; CELLS;
D O I：
10.3390/batteries6020025
中图分类号：
O646 [电化学、电解、磁化学];
学科分类号：
081704 ;
摘要：
Lithium-Ion batteries are used in ever more demanding applications regarding operating range and safety requirements. This work presents a series of high-temperature abuse experiments on a nickel-manganese-cobalt oxide (NMC)/graphite lithium-ion battery cell, using advanced in-operando measurement techniques like fast impedance spectroscopy and ultrasonic waves, as well as strain-gauges. the presented results show, that by using these methods degradation effects at elevated temperature can be observed in real-time. These methods have the potential to be integrated into a battery management system in the future. Therefore they make it possible to achieve higher battery safety even under the most demanding operating conditions.
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页数：20
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