Multiphase reacting flow studies of bubble column ozonation reactor for water remediation

被引:6
|
作者
Perdigoto, Marisa L. N. [1 ]
Larachi, Faical [2 ]
Lopes, Rodrigo J. G. [1 ]
机构
[1] Univ Coimbra, Dept Chem Engn, CIEPQPF, GERSE Grp Environm React & Separat Engn, P-3030790 Coimbra, Portugal
[2] Univ Laval, Dept Chem Engn, Quebec City, PQ G1K 7P4, Canada
关键词
Ethylene; Bubble column reactor; Electrical capacitance tomography; Hydrodynamics; Ozonation; Reactive flow; ELECTRICAL CAPACITANCE TOMOGRAPHY; COMPUTATIONAL FLUID-DYNAMICS; DISPERSED GAS/LIQUID FLOWS; LIQUID MASS-TRANSFER; NUMERICAL-SIMULATION; PART II; CFD; FILTRATION; MECHANISM;
D O I
10.1002/ceat.201200348
中图分类号
TQ [化学工业];
学科分类号
0817 ;
摘要
A multiphase Volume-of-fluid (VOF) model was developed to gain further insights into the reactive flow parameters and electrical capacitance tomography (ECT) measurements on the remediation of hazardous organic pollutants. Low ozone bubble frequencies were obtained for high surface tension fluids, and the liquid viscosity affected the ozone bubbling frequency. The VOF model indicated that the increase of inlet gas velocity enriched the ozone bubble detachment and concomitantly generated larger ozone bubbles, decreasing the detoxification rates. VOF mappings and ECT visualizations of gas-liquid unveiled preferential routes and highlighted the attenuation of the axisymmetric behavior of the ozonation bubble column under high-interaction regimes.
引用
收藏
页码:137 / 146
页数:10
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