Magnetic excitation spectrum of Na2IrO3 probed with resonant inelastic x-ray scattering

被引:82
|
作者
Gretarsson, H. [1 ]
Clancy, J. P. [1 ]
Singh, Yogesh [2 ]
Gegenwart, P. [3 ]
Hill, J. P. [4 ]
Kim, Jungho [5 ]
Upton, M. H. [5 ]
Said, A. H. [5 ]
Casa, D. [5 ]
Gog, T. [5 ]
Kim, Young-June [1 ]
机构
[1] Univ Toronto, Dept Phys, Toronto, ON M5S 1A7, Canada
[2] Indian Inst Sci Educ & Res Mohali, Manauli 140306, PO, India
[3] Univ Gottingen, Inst Phys 1, D-37077 Gottingen, Germany
[4] Brookhaven Natl Lab, Condensed Matter Phys & Mat Sci Dept, Upton, NY 11973 USA
[5] Argonne Natl Lab, Adv Photon Source, Argonne, IL 60439 USA
基金
加拿大自然科学与工程研究理事会;
关键词
D O I
10.1103/PhysRevB.87.220407
中图分类号
T [工业技术];
学科分类号
08 ;
摘要
The low energy excitations in Na2IrO3 have been investigated using resonant inelastic x-ray scattering (RIXS). A magnetic excitation branch can be resolved, whose dispersion reaches a maximum energy of about 35 meV at the Gamma point. The momentum dependence of the excitation energy is much larger along the Gamma-X direction compared to that along the Gamma-Y direction. The observed dispersion relation is consistent with a recent theoretical prediction based on the Heisenberg-Kitaev model. At high temperatures, we find large contributions from lattice vibrational modes to our RIXS spectra, suggesting that a strong electron-lattice coupling is present in Na2IrO3.
引用
收藏
页数:5
相关论文
共 50 条
  • [1] Resonant inelastic X-ray scattering spectra at the Ir L-edge in Na2IrO3
    Igarashi, Jun-ichi
    Nagao, Tatsuya
    JOURNAL OF ELECTRON SPECTROSCOPY AND RELATED PHENOMENA, 2016, 212 : 44 - 49
  • [2] Dynamic Spin Correlations in the Honeycomb Lattice Na2IrO3 Measured by Resonant Inelastic x-Ray Scattering
    Kim, Jungho
    Chaloupka, Jiri
    Singh, Yogesh
    Kim, J. W.
    Kim, B. J.
    Casa, D.
    Said, A.
    Huang, X.
    Gog, T.
    PHYSICAL REVIEW X, 2020, 10 (02):
  • [3] Magnetic Excitation Spectra of Sr2IrO4 Probed by Resonant Inelastic X-Ray Scattering: Establishing Links to Cuprate Superconductors
    Kim, Jungho
    Casa, D.
    Upton, M. H.
    Gog, T.
    Kim, Young-June
    Mitchell, J. F.
    van Veenendaal, M.
    Daghofer, M.
    van den Brink, J.
    Khaliullin, G.
    Kim, B. J.
    PHYSICAL REVIEW LETTERS, 2012, 108 (17)
  • [4] Magnetic excitation in resonant inelastic x-ray scattering of Sr2IrO4: A localized spin picture
    Igarashi, Jun-ichi
    Nagao, Tatsuya
    PHYSICAL REVIEW B, 2014, 89 (06)
  • [5] Ionic Solutions Probed by Resonant Inelastic X-ray Scattering
    Yin, Zhong
    Rajkovic, Ivan
    Veedu, Sreevidya Thekku
    Deinert, Sascha
    Raiser, Dirk
    Jain, Rohit
    Fukuzawa, Hironobu
    Wada, Shin-ichi
    Quevedo, Wilson
    Kennedy, Brian
    Schreck, Simon
    Pietzsch, Annette
    Wernet, Philippe
    Ueda, Kyoshi
    Foehlisch, Alexander
    Techert, Simone
    ZEITSCHRIFT FUR PHYSIKALISCHE CHEMIE-INTERNATIONAL JOURNAL OF RESEARCH IN PHYSICAL CHEMISTRY & CHEMICAL PHYSICS, 2015, 229 (10-12): : 1855 - 1867
  • [6] Chemical Reduction of Actinides Probed by Resonant Inelastic X-ray Scattering
    Butorin, Sergei M.
    Shuh, David K.
    Kvashnina, Kristina O.
    Guo, Jinghua
    Werme, Lars
    Nordgren, Joseph
    ANALYTICAL CHEMISTRY, 2013, 85 (23) : 11196 - 11200
  • [7] Excitation pathways in resonant inelastic x-ray scattering of solids
    Vorwerk, Christian
    Sottile, Francesco
    Draxl, Claudia
    PHYSICAL REVIEW RESEARCH, 2020, 2 (04):
  • [8] Magnetic circular dichroism in the dd excitation in the van der Waals magnet CrI3 probed by resonant inelastic x-ray scattering
    Ghosh, Anirudha
    Joensson, H. Johan M.
    Mukkattukavil, Deepak John
    Kvashnin, Yaroslav
    Phuyal, Dibya
    Thunstroem, Patrik
    Agaker, Marcus
    Nicolaou, Alessandro
    Jonak, Martin
    Klingeler, Ruediger
    Kamalakar, M. Venkata
    Sarkar, Tapati
    Vasiliev, Alexander N.
    Butorin, Sergei M.
    Eriksson, Olle
    Abdel-Hafiez, Mahmoud
    PHYSICAL REVIEW B, 2023, 107 (11)
  • [9] Magnetic excitations in La2CuO4 probed by indirect resonant inelastic x-ray scattering
    Forte, Filomena
    Ament, Luuk J. P.
    van den Brink, Jeroen
    PHYSICAL REVIEW B, 2008, 77 (13):
  • [10] Electronic structure of americium sesquioxide probed by resonant inelastic x-ray scattering
    Butorin, S. M.
    Shuh, D. K.
    PHYSICAL REVIEW B, 2023, 108 (19)