Emission of polycyclic aromatic hydrocarbons in China

被引:516
|
作者
Xu, SS [1 ]
Liu, WX [1 ]
Tao, S [1 ]
机构
[1] Peking Univ, Coll Environm Sci, Lab Earth Surface Proc, Beijing 100871, Peoples R China
关键词
D O I
10.1021/es0517062
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Emission of 16 polycyclic aromatic hydrocarbons (PAHs) listed as U.S. Environmental Protection Agency (U.S. EPA) priority pollutants from major sources in China were compiled. Geographical distribution and temporal change of the PAH emission, as well as emission profiles, are discussed. It was estimated that the total PAH emission in China was 25 300 tons in 2003. The emission profile featured a relatively higher portion of high molecular weight (HMW) species with carcinogenic potential due to large contributions of domestic coal and coking industry. Among various sources, biomass burning, domestic coal combustion, and coking industry contributed 60%, 20%, and 16% of the total emission, respectively. Total emission, emission density, emission intensity, and emission per capita showed geographical variations. In general, the southeastern provinces were characterized by higher emission density, while those in western and northern China featured higher emission intensity and population-normalized emission Although energy consumption in China went up continuously during the past two decades, annual emission of PAHs fluctuated depending on the amount of domestic coal consumption, coke production, and the efficiency of energy utilization.
引用
收藏
页码:702 / 708
页数:7
相关论文
共 50 条
  • [1] Emission of polycyclic aromatic hydrocarbons in China by county
    Zhang, Yanxu
    Tao, Shu
    Cao, Jun
    Coveney, Raymond M., Jr.
    [J]. ENVIRONMENTAL SCIENCE & TECHNOLOGY, 2007, 41 (03) : 683 - 687
  • [2] Emission and outflow of polycyclic aromatic hydrocarbons from wildfires in China
    Yuan, Huishi
    Tao, Shu
    Li, Bengang
    Lang, Chang
    Cao, Jun
    Coveney, Raymond M.
    [J]. ATMOSPHERIC ENVIRONMENT, 2008, 42 (28) : 6828 - 6835
  • [3] Emission, Fate and Exposure Risk of Polycyclic Aromatic Hydrocarbons in China
    Tao, Shu
    Zhang, Yanxu
    [J]. MOLECULAR ENVIRONMENTAL SOIL SCIENCE AT THE INTERFACES IN THE EARTH'S CRITICAL ZONE, 2010, : 293 - 293
  • [4] Emission factors of oxygenated polycyclic aromatic hydrocarbons from ships in China*
    Liang, Xuyang
    Wang, Lizhi
    Du, Wei
    Chen, Yuanchen
    Yun, Xiao
    Chen, Yilin
    Shen, Guofeng
    Shen, Huizhong
    Yang, Xin
    Tao, Shu
    [J]. ENVIRONMENTAL POLLUTION, 2023, 337
  • [5] Provincial emission inventory of atmospheric polycyclic aromatic hydrocarbons (PAHs) in China
    Wang, Jianbing
    Xia, Linlin
    Wang, Ruwei
    [J]. ATMOSPHERIC ENVIRONMENT, 2024, 334
  • [6] Survey of polycyclic aromatic hydrocarbons and nitrated polycyclic aromatic hydrocarbons in Jiaxing city, China
    Zhang, Yuejin
    Wang, Juan
    Ge, Zhigang
    Guo, Guanlin
    Gao, Shumei
    [J]. ENVIRONMENTAL EARTH SCIENCES, 2014, 71 (03) : 1095 - 1103
  • [7] Survey of polycyclic aromatic hydrocarbons and nitrated polycyclic aromatic hydrocarbons in Jiaxing city, China
    Yuejin Zhang
    Juan Wang
    Zhigang Ge
    Guanlin Guo
    Shumei Gao
    [J]. Environmental Earth Sciences, 2014, 71 : 1095 - 1103
  • [8] Emission factors of polycyclic aromatic hydrocarbons from domestic coal combustion in China
    Chunmei Geng
    Jianhua Chen
    Xiaoyang Yang
    Lihong Ren
    Baohui Yin
    Xiaoyu Liu
    Zhipeng Bai
    [J]. Journal of Environmental Sciences., 2014, 26 (01) - 166
  • [9] The Characteristics of Polycyclic Aromatic Hydrocarbons in Different Emission Source Areas in Shenyang, China
    Yang, Lu
    Suzuki, Genki
    Zhang, Lulu
    Zhou, Quanyu
    Zhang, Xuan
    Xing, Wanli
    Shima, Masayuki
    Yoda, Yoshiko
    Nakatsubo, Ryohei
    Hiraki, Takatoshi
    Sun, Baijun
    Fu, Wenhua
    Qi, Hongye
    Hayakawa, Kazuichi
    Toriba, Akira
    Tang, Ning
    [J]. INTERNATIONAL JOURNAL OF ENVIRONMENTAL RESEARCH AND PUBLIC HEALTH, 2019, 16 (16)
  • [10] Emission factors of polycyclic aromatic hydrocarbons from domestic coal combustion in China
    Chunmei Geng
    Jianhua Chen
    Xiaoyang Yang
    Lihong Ren
    Baohui Yin
    Xiaoyu Liu
    Zhipeng Bai
    [J]. Journal of Environmental Sciences, 2014, (01) : 160 - 166