Photochemical CO2 reduction in water using a co-immobilised nickel catalyst and a visible light sensitiser

被引：50

作者：

Neri, Gaia ^{[1
,2
]}

Forster, Mark ^{[1
,2
]}

Walsh, James J. ^{[1
,2
]}

Robertson, C. M. ^{[1
]}

Whittles, T. J. ^{[2
,3
]}

Farras, Pau ^{[4
]}

Cowan, Alexander J. ^{[1
,2
]}

机构：

[1] Univ Liverpool, Dept Chem, Liverpool L69 7ZD, Merseyside, England

[2] Univ Liverpool, Stephenson Inst Renewable Energy, Liverpool L69 7ZD, Merseyside, England

[3] Univ Liverpool, Dept Phys, Liverpool L69 7ZE, Merseyside, England

[4] Natl Univ Ireland Galway, Dept Chem, Galway, Ireland

来源：

CHEMICAL COMMUNICATIONS | 2016年 / 52卷 / 99期

基金：

英国工程与自然科学研究理事会;

关键词：

CARBON-DIOXIDE REDUCTION; HYBRID PHOTOCATALYST; MOLECULAR CATALYSTS; CYCLAM CYCLAM; COMPLEX; PHOTOREDUCTION; 1,4,8,11-TETRAAZACYCLOTETRADECANE; SYSTEM; ELECTRODES; INTERFACES;

D O I：

10.1039/c6cc08590c

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

A dye-sensitised CO2 reduction photocatalyst that operates in water is reported. Transient spectroscopy demonstrates that the facile co-immobilisation of a Ru dye and a Ni CO2 reduction electrocatalyst enables efficient on-particle electron transfer leading to photocatalytic activity that greatly exceeds the equivalent solution based system.

引用

页码：14200 / 14203

页数：4

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