Vibrational CARS thermometry and one-dimensional simulations in laminar H2/air counter-flow diffusion flames

被引:6
|
作者
Satija, Aman [1 ]
Huang, Xianan [1 ]
Panda, Pratikash P. [1 ]
Lucht, Robert P. [1 ]
机构
[1] Purdue Univ, Sch Mech Engn, W Lafayette, IN 47906 USA
关键词
CARS; Diffusion flame; Thermometry; Spectroscopy; STRAIN-INDUCED EXTINCTION; COMBUSTION; TEMPERATURE; PRESSURE; LIMITS;
D O I
10.1016/j.ijhydene.2015.06.150
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Broadband N-2 vibrational coherent anti-Stokes Raman scattering (VCARS) thermometry was performed along the nozzle centerline of counter-flow diffusion flames. Fuel mixtures consisted of varying percentages of H-2 in N-2 and the oxidizer was air. We investigated the influence of varying the percentage of H-2 in the fuel stream on the temperature profiles along the nozzle centerline. Measurements were performed, with varying global strain rates, both near and far from flame extinction. One-dimensional simulations, performed using Combustion Simulation Lab (COSILAB) software, show that the temperature profiles are relatively insensitive to the nozzle exit centerline velocity; implying that the 1-D simulations provide an excellent approximation of the real temperature profiles along the nozzle centerline. Various chemical mechanisms were employed within the COSILAB framework for comparison against VCARS temperature measurements. Simulations were also performed to evaluate the influence of thermal diffusion and nitrogen chemistry on nozzle centerline temperature profiles. Copyright (C) 2015, Hydrogen Energy Publications, LLC. Published by Elsevier Ltd. All rights reserved.
引用
收藏
页码:10662 / 10672
页数:11
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