Cavitation bubble dynamics and sonochemiluminescence activity inside sonicated submerged flow tubes

被引:12
|
作者
Sarac, Busra Ekim [1 ]
Stephens, Dwayne Savio [1 ]
Eisener, Julian [1 ,2 ]
Rossello, Juan Manuel [1 ]
Mettin, Robert [1 ]
机构
[1] Georg August Univ Gottingen, Drittes Phys Inst, Friedrich Hund Pl 1, D-37077 Gottingen, Germany
[2] Otto von Guericke Univ, Inst Phys, Univ Pl 2, D-39106 Magdeburg, Germany
基金
欧盟地平线“2020”;
关键词
Sonochemistry; Luminol; Ultrasound; Nucleation; High-speed observations; Bubble dynamics; ULTRASOUND PROPAGATION; SIMPLE-MODEL; SONOCHEMISTRY; SONOLUMINESCENCE; INTENSIFICATION; MICROFLUIDICS; MICROREACTOR; POPULATIONS; ENERGY;
D O I
10.1016/j.cep.2020.107872
中图分类号
TE [石油、天然气工业]; TK [能源与动力工程];
学科分类号
0807 ; 0820 ;
摘要
Bubble dynamics and luminol emissions of cavitation in sub-millimeter-sized perfluoroalkoxy alkane (PFA) flow tubes, submerged in an ultrasonic bath reactor, are studied at 27.2 kHz driving frequency. Nucleation of cavitation inside the tubes only takes place via a free interface, realized here in form of an alternating water-air slug flow. High-speed recordings show that cavitation bubbles in the water slugs often develop localized structures in form of clusters or bubble "plugs", and that such structures can be seeded via a single pinch-off from the free interface. Within the structures, bubbles strongly interact and frequently undergo merging or splitting events. Due to the mutual interaction and resulting motion, bubbles often collapse with a fast displacement, suggesting jetting dynamics. Bubble compression ratios are estimated on basis of observed individual bubble dynamics and numerical fitting by a single bubble model that takes the tube wall into account. The resulting peak temperatures around 3500 K allow for dissociation of water vapor. This is in accordance with observed sonochemiluminescence from luminol, originating from active bubble zones in the tubes.
引用
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页数:9
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