Scalable One-Step Assembly of an Inexpensive Photoelectrode for Water Oxidation by Deposition of a Ti- and Ni-Containing Molecular Precursor on Nanostructured WO3

被引：33

作者：

Lai, Yi-Hsuan ^{[1
]}

King, Timothy C. ^{[1
]}

Wright, Dominic S. ^{[1
]}

Reisner, Erwin ^{[1
]}

机构：

[1] Univ Cambridge, Dept Chem, Christian Doppler Lab Sustainable SynGas Chem, Cambridge CB2 1EW, England

来源：

CHEMISTRY-A EUROPEAN JOURNAL | 2013年 / 19卷 / 39期

基金：

英国工程与自然科学研究理事会;

关键词：

photochemistry; photooxidation; photosynthesis; water oxidation; water splitting; VISIBLE-LIGHT; TUNGSTEN TRIOXIDE; OXYGEN EVOLUTION; HYDROGEN-PRODUCTION; PHOTOSYSTEM-II; PHOTOANODES; FILMS; CATALYSTS; TITANIUM; PHOTOOXIDATION;

D O I：

10.1002/chem.201302641

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Photoactive in one step! A nanocomposite water-oxidation photocatalyst was assembled by a straightforward and one-step spin-coating procedure of a Ti- and Ni-containing molecule on nanostructured WO3. The photoanode oxidizes water to O2 with good activity and stability in alkaline solution, and thereby features light absorption, charge separation and water-oxidation catalysis (see scheme). © 2013 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.

引用

下载

页码：12943 / 12947

页数：5