Facile Synthesis of a Phosphorylcholine-Based Zwitterionic Amphiphilic Copolymer for Anti-Biofouling Coatings

被引：28

作者：

Seetho, Kellie ^{[1
,2
,3
]}

Zhang, Shiyi ^{[1
,2
,3
]}

Pollack, Kevin A. ^{[1
,2
,3
]}

Zou, Jiong ^{[1
,2
,3
]}

Raymond, Jeffery E. ^{[1
,2
,3
]}

Martinez, Edgar ^{[4
]}

Wooley, Karen L. ^{[1
,2
,3
]}

机构：

[1] Texas A&M Univ, Lab Synthet Biol Interact, Dept Chem, College Stn, TX 77842 USA

[2] Texas A&M Univ, Lab Synthet Biol Interact, Dept Chem Engn, College Stn, TX 77842 USA

[3] Texas A&M Univ, Lab Synthet Biol Interact, Dept Mat Sci & Engn, College Stn, TX 77842 USA

[4] Beclunan Coulter Particle Characterizat Lab, Miami, FL 33196 USA

来源：

ACS MACRO LETTERS | 2015年 / 4卷 / 05期

关键词：

PHOSPHOLIPID POLYMERS; PROTEIN ADSORPTION; SURFACE; MARINE; RESISTANCE; ROUGHNESS;

D O I：

10.1021/mz500818c

中图分类号：

O63 [高分子化学（高聚物）];

学科分类号：

070305 ; 080501 ; 081704 ;

摘要：

An antibiofouling polymer coating, combined with both zwitterionic and amphiphilic features, is engineered by a two-step modification of a commodity polymer. The surface properties of the resultant polymer coating can be easily tuned by varying the extent of cross-linking in the network. Higher antibiofouling efficiency was observed for these surfaces vs. an elastomeric polydimethylsiloxane standard (Sylgard 184) against the adsorption of biomacromolecules and a marine fouling organism (Ulva zoospores) has been demonstrated. This design establishes a platform for the achievement of functionalized amphiphilic zwitterionic copolymers from relatively inexpensive starting materials via simple chemical manipulations.

引用

页码：505 / 510

页数：6

共 50 条

[1] Anti-biofouling properties of amphiphilic phosphorylcholine polymer films
Li, Yan
Liu, Cheng-Mei
Yang, Jin-Ying
Gao, Ya-Hui
Li, Xue-Song
Que, Guo-He
Lu, J. R.
[J]. COLLOIDS AND SURFACES B-BIOINTERFACES, 2011, 85 (02) : 125 - 130
[2] Synthesis and anti-biofouling studies of a novel amphiphilic zwitterionic polymeric system
Seetho, Kellie
Zhang, Shiyi
Raymond, Jeffery E.
Wang, Hai
Wooley, Karen L.
[J]. ABSTRACTS OF PAPERS OF THE AMERICAN CHEMICAL SOCIETY, 2013, 246
[3] Amphiphilic Copolymer Coatings via Plasma Polymerisation Process: Switching and Anti-Biofouling Characteristics
Kumar, Virendra
Pulpytel, Jerome
Giudetti, Guido
Rauscher, Hubert
Rossi, Francois
Arefi-Khonsari, Farzaneh
[J]. PLASMA PROCESSES AND POLYMERS, 2011, 8 (05) : 373 - 385
[4] Synthesis and Characterization of a Novel Amphiphilic Copolymer Capable as Anti-Biofouling Coating Material
Feng, Shijun
Wang, Qiang
Gao, Yu
Huang, Yangen
Qing, Feng-Ling
[J]. JOURNAL OF APPLIED POLYMER SCIENCE, 2009, 114 (04) : 2071 - 2078
[5] Revealing Amphiphilic Nanodornains of Anti-Biofouling Polymer Coatings
Amadei, Carlo A.
Yang, Rong
Chiesa, Matteo
Gleason, Karen K.
Santos, Sergio
[J]. ACS APPLIED MATERIALS & INTERFACES, 2014, 6 (07) : 4705 - 4712
[6] Fabrication and Characterization of Zwitterionic Coatings with Anti-oil and Anti-biofouling Activities
Wu, Ruijie
Li, Lin
Dong, Guangli
Qin, Yanqiong
Li, Mingwei
Hao, Hong
[J]. JOURNAL OF MACROMOLECULAR SCIENCE PART B-PHYSICS, 2022, 61 (06): : 825 - 843
[7] Phosphorylcholine-Based Zwitterionic Biocompatible Thermogel
Ko, Du Young
Patel, Madhumita
Jung, Bo Kyoeng
Park, Jin Hye
Jeong, Byeongmoon
[J]. BIOMACROMOLECULES, 2015, 16 (12) : 3853 - 3862
[8] Water-repairable zwitterionic polymer coatings for anti-biofouling surfacese
Wang, Zhanhua
van Andel, Esther
Pujari, Sidharam P.
Feng, Huanhuan
Dijksman, Joshua A.
Smulders, Maarten M. J.
Zuilhof, Han
[J]. JOURNAL OF MATERIALS CHEMISTRY B, 2017, 5 (33) : 6728 - 6733
[9] Phosphorylcholine-based polymers and their use in the prevention of biofouling
Lewis, AL
[J]. COLLOIDS AND SURFACES B-BIOINTERFACES, 2000, 18 (3-4) : 261 - 275
[10] Dual water-healable zwitterionic polymer coatings for anti-biofouling surfaces
Wang, Zhanhua
Fei, Guoxia
Xia, Hesheng
Zuilhof, Han
[J]. JOURNAL OF MATERIALS CHEMISTRY B, 2018, 6 (43) : 6930 - 6935

← 1 2 3 4 5 →