Bioenergy potential of Wolffia arrhiza appraised through pyrolysis, kinetics, thermodynamics parameters and TG-FTIR-MS study of the evolved gases

被引:98
|
作者
Ahmad, Muhammad Sajjad [2 ]
Mehmood, Muhammad Aamer [1 ,2 ]
Liu, Chen-Guang [3 ]
Tawab, Abdul [4 ]
Bai, Feng-Wu [3 ]
Sakdaronnarong, Chularat [5 ]
Xu, Jianren [3 ]
Rahimuddin, Sawsan Abdulaziz [6 ]
Gull, Munazza [6 ]
机构
[1] Sichuan Univ Sci & Engn, Coll Bioengn, Zigong 643000, Peoples R China
[2] Univ Faisalabad, Govt Coll, Dept Bioinformat & Biotechnol, Bioenergy Res Ctr, Faisalabad 38000, Pakistan
[3] Shanghai Jiao Tong Univ, Sch Life Sci & Biotechnol, State Key Lab Microbial Metab, Shanghai 200240, Peoples R China
[4] Natl Inst Biotechnol & Genet Engn, Faisalabad 38000, Pakistan
[5] Mahidol Univ, Dept Chem Engn, Phutthamonthon 73170, Nakhon Pathom, Thailand
[6] King Abdulaziz Univ, Fac Sci, Biochem Dept, Jeddah 21551, Saudi Arabia
基金
中国国家自然科学基金;
关键词
Wolffia biomass; Pyrolysis; TG-FTIR-MS; Bioenergy; Waste-to-fuel; THERMOGRAVIMETRIC ANALYSIS; BIOMASS; GRASS; COMBUSTION; MANURE; WASTE; DECOMPOSITION; BEHAVIOR; ENERGY; ARUNDO;
D O I
10.1016/j.biortech.2018.01.033
中图分类号
S2 [农业工程];
学科分类号
0828 ;
摘要
This study evaluated the bioenergy potential of Wolffia arrhiza via pyrolysis. The biomass was collected from the pond receiving city wastewater. Oven dried powdered biomass was exposed to thermal degradation at three heating rates (10, 30 and 50 degrees C min(-1)) using Thermogravimetry-Differential Scanning Calorimetry analyzer in an inert environment. Data obtained were subjected to the isoconversional models of Kissenger-Akahira-Sunose (KSA) and Flynn-Wall-Ozawa (FWO) to elucidate the reaction chemistry. Kinetic parameters including, Ea (136-172 kJmol(-1)) and Gibb's free energy (171 kJmol(-1)) showed the remarkable bioenergy potential of the biomass. The average enthalpies indicated that the product formation is favored during pyrolysis. Advanced coupled TG-FTIR-MS analyses showed the evolved gases to contain the compounds containing C-O functional groups (aldehydes, ketones), aromatic and aliphatic hydrocarbons as major pyrolytic products. This low-cost abundant biomass may be used to produce energy and chemicals in a cost-efficient and environmentally friendly way.
引用
收藏
页码:297 / 303
页数:7
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