Combined treatment of hydroxypropyl guar gum in oilfield fracturing wastewater by coagulation and the UV/H2O2/ferrioxalate complexes process

被引:7
|
作者
Zhang, Zhenchao [1 ]
机构
[1] Northeast Petr Univ, Coll Chem & Chem Engn, Daqing 163318, Peoples R China
关键词
coagulation process; hydroxypropyl guar gum; oilfield fracturing wastewater; UV/H2O2/ferrioxalate complexes process; UV-vis spectra analysis; PHOTO-FENTON DEGRADATION; LANDFILL LEACHATE; ORGANIC CONTAMINANTS; FERRIOXALATE COMPLEX; STABILIZED LEACHATE; OXIDATION; REMOVAL; FLOCCULATION; COD; PRETREATMENT;
D O I
10.2166/wst.2017.552
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Hydroxypropyl guar gum is considered to be a main component of oilfield fracturing wastewater (OFW). This work is intended to optimize the experimental conditions for the maximum oxidative degradation of hydroxypropyl guar gum by the coagulation and UV/H2O2/ferrioxalate complexes process. Optimal reaction conditions were proposed based on the chemical oxygen demand (COD) removal efficiency and UV-vis spectra analysis. The overall removal efficiency of COD reached 83.8% for a dilution ratio of raw wastewater of 1: 2, pH of 4 and FeCl3 loading of 1,000 mg/L in the coagulation process; the dosage of H2O2 (30%, v/v) was 0.6% (v/v) and added in three steps, the n(H2O2)/n(Fe2+) was 2: 1, n(Fe2+)/n(C2O42-) was 3: 1 and pH was 4 in the UV/H2O2/ferrioxalate complexes process; pH was adjusted to 8.5-9 by NaOH and then cationic polyacrylamide (CPAM) of 2 mg/L was added in the neutralization and flocculation process. The decrease in COD during the coagulation process reduced the required H2O2 dosage and improved efficiency in the subsequent UV/H2O2/ferrioxalate complexes process. Furthermore, COD removal efficiency significantly increased by more than 13.4% with the introduction of oxalate compared with UV/Fenton. The UV-vis spectra analysis results indicated that the coagulation and UV/H2O2/ferrioxalate complexes process could efficiently remove the hydroxypropyl guar gum dissolved in OFW. An optimal combination of these parameters produced treated wastewater that met the GB8978-1996 Integrated Wastewater Discharge Standard level III emission standard.
引用
收藏
页码:565 / 575
页数:11
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