Quantum coherent control of two-photon transitions by square phase-modulation

被引：7
|
作者：
Zhang Shi-An [1 ]
Wang Zu-Geng [1 ]
Sun Zhen-Rong [1 ]
机构：
[1] E China Normal Univ, Dept Phys, State Key Lab Precis Spect, Shanghai 200062, Peoples R China
来源：
CHINESE PHYSICS B | 2008年 / 17卷 / 08期
基金：
中国国家自然科学基金;
关键词：
two-photon transitions; coherent control; pulse shaping;
D O I：
10.1088/1674-1056/17/8/026
中图分类号：
O4 [物理学];
学科分类号：
0702 ;
摘要：
A femtosecond laser pulse can be tailored to control the two-photon transitions using the ultra-fast pulse-shaping technique. This paper theoretically and experimentally demonstrates that two-photon transitions in molecular system with broad absorption line can be effectively controlled by square phase-modulation in frequency domain, and the influence of all parameters characterizing the square phase-modulation on two-photon transitions is systemically investigated and discussed. The obtained results have potential application in nonlinear spectroscopy and molecular physics.
引用
收藏
页码：2914 / 2918
页数：5
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