A Water Stable Metal-Organic Framework with Optimal Features for CO2 Capture

被引：312

作者：

Yang, Qingyuan ^{[1
]}

Vaesen, Sebastien ^{[2
]}

Ragon, Florence ^{[4
]}

Wiersum, Andrew D. ^{[3
]}

Wu, Dong ^{[1
]}

Lago, Ana ^{[4
]}

Devic, Thomas ^{[4
]}

Martineau, Charlotte ^{[4
]}

Taulelle, Francis ^{[4
]}

Llewellyn, Philip L. ^{[3
]}

Jobic, Herve ^{[5
]}

Zhong, Chongli ^{[1
]}

Serre, Christian ^{[4
]}

De Weireld, Guy ^{[2
]}

Maurin, Guillaume ^{[6
]}

机构：

[1] Beijing Univ Chem Technol, State Key Lab Organ Inorgan Composites, Beijing 100029, Peoples R China

[2] Univ Mons, Thermodynam Dept, Fac Polytech, B-7000 Mons, Belgium

[3] Aix Marseille Univ, Lab MADIREL, CNRS, UMR 7246,Ctr St Jerome, F-13397 Marseille, France

[4] Univ Versailles, CNRS, UMR 8180, Inst Lavoisier, F-78035 Versailles, France

[5] Univ Lyon, CNRS, Inst Rech Catalyse & Environm Lyon, F-69626 Villeurbanne, France

[6] UM2, ENSCM, CNRS, Inst Charles Gerhardt Montpellier,UMR 5253, F-34095 Montpellier 05, France

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2013年 / 52卷 / 39期

关键词：

CO2; separation; flue gas; green synthesis; metal-organic frameworks; zirconium; ZIRCONIUM TEREPHTHALATE UIO-66(ZR); ELASTIC NEUTRON-SCATTERING; CARBON-DIOXIDE CAPTURE; MICROPOROUS COORDINATION POLYMERS; MOLECULAR-DYNAMICS; GAS-MIXTURE; ZEOLITE; 13X; PORE-SIZE; ADSORPTION; METHANE;

D O I：

10.1002/anie.201302682

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

One flue over the cuckoo's nest: A novel porous Zr-based MOF combining a high chemical stability, easy "green" synthesis and scalability is prepared. This material incorporating carboxylic functions on its organic linkers has thermodynamically and kinetically very promising properties for CO2 capture from post-combustion flue gas under real working conditions. Copyright © 2013 WILEY-VCH Verlag GmbH & Co. KGaA, Weinheim.

引用

页码：10316 / 10320

页数：5

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