Phase-matched third-harmonic generation in mercury-(I)-chloride

被引：7
|
作者：
Schmitzer, H [1 ]
Wagner, HP
Dultz, W
Kühnelt, M
机构：
[1] TU Chemnitz, Inst Phys, D-09107 Chemnitz, Germany
[2] Univ Cincinnati, Cincinnati, OH 45221 USA
[3] Goethe Univ Frankfurt, D-60054 Frankfurt, Germany
[4] Osram Opto Semicond, D-093049 Regensburg, Germany
来源：
APPLIED OPTICS | 2002年 / 41卷 / 03期
关键词：
D O I：
10.1364/AO.41.000470
中图分类号：
O43 [光学];
学科分类号：
070207 ; 0803 ;
摘要：
Using phase-matched third-harmonic generation we determine the effective nonlinear susceptibilities in Hg2Cl2 (Calomel) to \chi(eff,I)((3))\ = 4.5 x 10(-22) m(2)V(-2) and \chi(eff,II)((3))\ = 9.7 x 10(-22)m(2)V(-2) for type I and type II phase matching, respectively. The type III phase matching uses the same tensor components as type I and is deduced to be \chi(eff,III)((3))\ congruent to 1.5 x 10(-22)m(2)V(-2). The effective third-order susceptibilities of Hg2Cl2 are two orders of magnitude higher than those of CaCO3 and the tensor components chi(11) - 3chi(18) exceed the components of ADP by a factor of 5. These measurements demonstrate that Calomel might be a promising material to be used for nonlinear optical devices. (C) 2002 Optical Society of America.
引用
收藏
页码：470 / 474
页数：5
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