Anomalous diffusion and power-law relaxation of the time averaged mean squared displacement in worm-like micellar solutions

被引:221
|
作者
Jeon, Jae-Hyung [1 ]
Leijnse, Natascha [2 ]
Oddershede, Lene B. [2 ]
Metzler, Ralf [1 ,3 ]
机构
[1] Tampere Univ Technol, Dept Phys, FIN-33101 Tampere, Finland
[2] Univ Copenhagen, Niels Bohr Inst, DK-2100 Copenhagen O, Denmark
[3] Univ Potsdam, Inst Phys & Astron, D-14476 Potsdam, Germany
来源
NEW JOURNAL OF PHYSICS | 2013年 / 15卷
基金
芬兰科学院;
关键词
BIOLOGY; MOTION; MODELS; POINT;
D O I
10.1088/1367-2630/15/4/045011
中图分类号
O4 [物理学];
学科分类号
0702 ;
摘要
We report the results of single tracer particle tracking by optical tweezers and video microscopy in micellar solutions. From careful analysis in terms of different stochastic models, we show that the polystyrene tracer beads of size 0.52-2.5 mu m after short-time normal diffusion turn over to perform anomalous diffusion of the form < r(2)(t)> similar or equal to t(alpha) with alpha approximate to 0.3. This free anomalous diffusion is ergodic and consistent with a description in terms of the generalized Langevin equation with a power-law memory kernel. With optical tweezers tracking, we unveil a power-law relaxation over several decades in time to the thermal plateau value under the confinement of the harmonic tweezer potential, as predicted previously (Phys. Rev. E 85 021147 (2012)). After the subdiffusive motion in the millisecond range, the motion becomes faster and turns either back to normal Brownian diffusion or to even faster superdiffusion, depending on the size of the tracer beads.
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页数:16
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