Low-Temperature Solution Processing of Mesoporous Metal-Sulfide Semiconductors as Light-Harvesting Photoanodes

被引：23

作者：

O'Mahony, Flannan T. F. ^{[1
]}

Cappel, Ute B. ^{[1
]}

Tokmoldin, Nurlan ^{[1
]}

Lutz, Thierry ^{[1
]}

Lindblad, Rebecka ^{[2
]}

Rensmo, Hakan ^{[2
]}

Haque, Saif A. ^{[1
]}

机构：

[1] Univ London Imperial Coll Sci Technol & Med, Dept Chem, Ctr Plast Elect, London SW7 2AZ, England

[2] Uppsala Univ, Dept Phys & Astron, S-75120 Uppsala, Sweden

来源：

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION | 2013年 / 52卷 / 46期

基金：

英国工程与自然科学研究理事会; 瑞典研究理事会;

关键词：

antimony; energy conversion; metal xanthates; nanostructures; time-resolved spectroscopy; SOLAR-CELL; SOLID-STATE; LOW-COST; FILMS; XANTHATES; ELECTRON; GROWTH; ROUTE;

D O I：

10.1002/anie.201305276

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

Structured absorbers: Mesoporous films of highly crystalline Sb 2S3 are prepared from a doctor-bladed precursor paste that is thermally annealed. This facile and versatile processing route allows for control of the pore size through variation of the annealing temperature. The resulting high surface area allows for efficient charge transfer to a polymeric hole acceptor; hence, such films could form the basis of a novel hybrid organic-inorganic photovoltaic device. © 2013 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA. This is an open access article under the terms of the Creative Commons Attribution License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.

引用

页码：12047 / 12051

页数：5

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