Novel MoS2quantum dots as a highly efficient visible-light driven photocatalyst in water remediation

被引:15
|
作者
Chen, Linjer [1 ]
Hsieh, Shu-Ling [2 ]
Kuo, Chia-Hung [2 ]
Hsieh, Shuchen [3 ,4 ]
Chen, Wei-Hsiang [5 ]
Chen, Chiu-Wen [1 ]
Dong, Cheng-Di [1 ]
机构
[1] Natl Kaohsiung Univ Sci & Technol, Dept Marine Environm Engn, Kaohsiung, Taiwan
[2] Natl Kaohsiung Marine Univ, Dept Seafood Sci, Kaohsiung 81157, Taiwan
[3] Natl Sun Yat Sen Univ, Dept Chem, 70 Lien Hai Rd, Kaohsiung 80424, Taiwan
[4] Natl Sun Yat Sen Univ, Ctr Nanosci & Nanotechnol, 70 Lien Hai Rd, Kaohsiung 80424, Taiwan
[5] Natl Sun Yat Sen Univ, Inst Environm Engn, Kaohsiung 804, Taiwan
关键词
PERFORMANCE; ENHANCEMENT; COMPOSITES; SHEETS;
D O I
10.1039/d0ra04512h
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
A direct and efficient hydrothermal system has been established for the synthesis of MoS(2)quantum dots (QDs). Novel MoS(2)QDs are an excellent potential photocatalysts to enhance photocatalytic response by charge separation under visible light irradiation. The optimum capability of QDs demonstrated the excellent photocatalytic ability for the degradation of organic pollutants. The microstructural, morphological, and optical properties of the MoS(2)QDs are definedviaX-ray diffraction (XRD), SEM, HRTEM, XPS, and UV-Vis absorption spectroscopy techniques. Under visible light irradiation, MoS(2)QDs have great photocatalytic response for the degradation of Rh B that is 20 times higher than those of bulk MoS(2)materials. The QDs possess practically the same catalytic response after 5 recycle runs, which is an evident proof of its stability. This course might pave the route toward creating current visible-light caused QD photocatalyst strategies for the highly valuable degradation of organic pollutants or antibiotics.
引用
收藏
页码:31794 / 31799
页数:6
相关论文
共 50 条
  • [1] MoS2-mesoporous LaFeO3 hybrid photocatalyst: Highly efficient visible-light driven photocatalyst
    Acharya, S.
    Swain, G.
    Parida, K. M.
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2020, 45 (20) : 11502 - 11511
  • [2] Phosphorus quantum dots as visible-light photocatalyst for water splitting
    Zhou, Si
    Liu, Nanshu
    Zhao, Jijun
    [J]. COMPUTATIONAL MATERIALS SCIENCE, 2017, 130 : 56 - 63
  • [3] Interface of GO with SnO2 quantum dots as an efficient visible-light photocatalyst
    Sahu, Binaya Kumar
    Juine, Rabindra Nath
    Sahoo, Madhusmita
    Kumar, Ravi
    Das, A.
    [J]. CHEMOSPHERE, 2021, 276
  • [4] Hybrid of AgInZnS and MoS2 as efficient visible-light driven photocatalyst for hydrogen production
    Huang, Ting
    Chen, Wei
    Liu, Tian-Yu
    Hao, Qing-Li
    Liu, Xiao-Heng
    [J]. INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (17) : 12254 - 12261
  • [5] A Dinuclear Cobalt Cryptate as a Photocatalyst for Highly Efficient Visible-Light Driven CO2 Reduction
    Lan Zhi-An
    Wang Xin-Chen
    [J]. ACTA PHYSICO-CHIMICA SINICA, 2017, 33 (03) : 457 - 457
  • [6] Visible-Light Driven TiO2 Photocatalyst Coated with Graphene Quantum Dots of Tunable Nitrogen Doping
    Sun, Xiong
    Li, Hui-Jun
    Ou, Nanquan
    Lyu, Bowen
    Gui, Bojie
    Tian, Shiwei
    Qian, Dongjin
    Wang, Xianying
    Yang, Junhe
    [J]. MOLECULES, 2019, 24 (02)
  • [7] Construction of Cu2O/Cu heterojunction with hierarchical hollow sphere structure as visible-light driven photocatalyst for efficient water remediation
    Li, Junhua
    Huang, Linsen
    Yang, Zhimei
    Liu, Zengjian
    Sun, Xiaosong
    [J]. JOURNAL OF ENVIRONMENTAL CHEMICAL ENGINEERING, 2022, 10 (03):
  • [8] Graphene quantum dots/BiOCl visible-light active photocatalyst for degradation of NO
    Nie, Qianqian
    Jia, Liuhu
    Luan, Jianfu
    Cui, Yunpei
    Liu, Jiayou
    Tan, Zhongchao
    Yu, Hesheng
    [J]. CHEMICAL ENGINEERING SCIENCE, 2024, 285
  • [9] Promising visible-light driven hydrogen production from water on a highly efficient CuCo2S4 nanosheet photocatalyst
    Chauhan, Meenakshi
    Soni, Kiran
    Karthik, P. E.
    Reddy, Kasala Prabhakar
    Gopinath, Chinnakonda S.
    Deka, Sasanka
    [J]. JOURNAL OF MATERIALS CHEMISTRY A, 2019, 7 (12) : 6985 - 6994
  • [10] ZnSe quantum dots modified with a Ni(cyclam) catalyst for efficient visible-light driven CO2 reduction in water
    Kuehnel, Moritz F.
    Sahm, Constantin D.
    Neri, Gaia
    Lee, Jonathan R.
    Orchard, Katherine L.
    Cowan, Alexander J.
    Reisner, Erwin
    [J]. CHEMICAL SCIENCE, 2018, 9 (09) : 2501 - 2509