Hierarchically macro-meso-microporous metal-organic framework for photocatalytic oxidation

被引：12

作者：

Sha, Yufei ^{[1
,2
]}

Zhang, Jianling ^{[1
,2
,3
]}

Tan, Dongxing ^{[1
,2
]}

Zhang, Fanyu ^{[1
,2
]}

Cheng, Xiuyan ^{[1
,2
]}

Tan, Xiuniang ^{[1
,2
]}

Zhang, Bingxing ^{[1
,2
]}

Han, Buxing ^{[1
,2
,3
]}

Zheng, Lirong ^{[4
]}

Zhang, Jing ^{[4
]}

机构：

[1] Chinese Acad Sci, Inst Chem, CAS Res Educ Ctr Excellence Mol Sci, Beijing Natl Lab Mol Sci,CAS Key Lab Colloid Inte, Beijing 100190, Peoples R China

[2] Univ Chinese Acad Sci, Sch Chem Sci, Beijing 100049, Peoples R China

[3] Huairou Natl Comprehens Sci Ctr, Phys Sci Lab, Beijing 101400, Peoples R China

[4] Chinese Acad Sci, Inst High Energy Phys, Beijing Synchrotron Radiat Facil BSRF, Beijing 100049, Peoples R China

来源：

CHEMICAL COMMUNICATIONS | 2020年 / 56卷 / 73期

基金：

中国国家自然科学基金;

关键词：

VISIBLE-LIGHT; AMINES; NANOSHEETS; REDUCTION; EFFICIENT; COMPLEX; IMINES; MOFS; XPS;

D O I：

10.1039/d0cc04389c

中图分类号：

O6 [化学];

学科分类号：

0703 ;

摘要：

The macro-meso-microporous and defective metal-organic framework constructed by transition metal Zn and 2,2 '-bipyridine-5,5 '-carboxylate was synthesized in CO2-expanded solvent. It shows high photocatalytic activity and selectivity for the oxidation of amines to imines under mild conditions,i.e., air as an oxidant, room temperature, and involving no photosensitizer or cocatalyst.

引用

页码：10754 / 10757

页数：4

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