Stimulated X-ray Raman scattering - a critical assessment of the building block of nonlinear X-ray spectroscopy

被引：19

作者：

Kimberg, Victor ^{[1
,2
]}

Sanchez-Gonzalez, Alvaro ^{[3
]}

Mercadier, Laurent ^{[1
]}

Weninger, Clemens ^{[1
,4
]}

Lutman, Alberto ^{[4
]}

Ratner, Daniel ^{[4
]}

Coffee, Ryan ^{[4
]}

Bucher, Maximilian ^{[4
,6
]}

Mucke, Melanie ^{[5
]}

Agaker, Marcus ^{[5
]}

Sathe, Conny ^{[5
]}

Bostedt, Christoph ^{[6
]}

Nordgren, Joseph ^{[5
]}

Rubensson, Jan Erik ^{[5
]}

Rohringer, Nina ^{[1
]}

机构：

[1] Max Planck Inst Struct & Dynam Matter, Hamburg, Germany

[2] Royal Inst Technol, Stockholm, Sweden

[3] Imperial Coll, Dept Phys, London, England

[4] SLAC Natl Accelerator Lab, LCLS, Menlo Pk, CA USA

[5] Uppsala Univ, Dept Phys & Astron, Uppsala, Sweden

[6] Argonne Natl Lab, Argonne, IL 60439 USA

来源：

FARADAY DISCUSSIONS | 2016年 / 194卷

基金：

瑞典研究理事会; 英国科学技术设施理事会;

关键词：

SPECTRA;

D O I：

10.1039/c6fd00103c

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

With the invention of femtosecond X-ray free-electron lasers (XFELs), studies of light-induced chemical reaction dynamics and structural dynamics reach a new era, allowing for time-resolved X-ray diffraction and spectroscopy. To ultimately probe coherent electron and nuclear dynamics on their natural time and length scales, coherent nonlinear X-ray spectroscopy schemes have been proposed. In this contribution, we want to critically assess the experimental realisation of nonlinear X-ray spectroscopy at current-day XFEL sources, by presenting first experimental attempts to demonstrate stimulated resonant X-ray Raman scattering in molecular gas targets.

引用

页码：305 / 324

页数：20

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