The effect of increasing fossil fuel combustion in eastern Asia on surface O-3 air pollution in the United States is examined with a global three-dimensional tropospheric chemistry model. Tripling of Asian anthropogenic emissions from 1985 to 2010 is expected to increase monthly mean O-3 concentrations by 2-6 ppbv in the western United States and by 1-3 ppbv in the eastern United States, the maximum effect being in April-June. This increase would more than offset the benefits of 25% domestic reductions in anthropogenic emissions of NOx and hydrocarbons in the western United States. Asian influence may be less under the stagnant conditions leading to violations of the U.S. air quality standard. Nevertheless, our results suggest that a global perspective is necessary when designing a strategy to meet regional O-3 air quality objectives.
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US EPA, Natl Exposure Res Lab, Atmospher Modeling Div, Res Triangle Pk, NC 27711 USAUS EPA, Natl Exposure Res Lab, Atmospher Modeling Div, Res Triangle Pk, NC 27711 USA
Sarwar, Golam
Bhave, Prakash V.
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US EPA, Natl Exposure Res Lab, Atmospher Modeling Div, Res Triangle Pk, NC 27711 USAUS EPA, Natl Exposure Res Lab, Atmospher Modeling Div, Res Triangle Pk, NC 27711 USA
机构:
Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
NOAA Earth Syst Res Lab, Boulder, CO 80305 USAPrinceton Univ, Princeton, NJ 08540 USA
Cooper, Owen R.
Naik, Vaishali
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High Performance Technol Inc, NOAA Geophys Fluid Dynam Lab, Princeton, NJ 08540 USAPrinceton Univ, Princeton, NJ 08540 USA
Naik, Vaishali
Holloway, John
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NOAA Earth Syst Res Lab, Boulder, CO 80305 USAPrinceton Univ, Princeton, NJ 08540 USA
Holloway, John
Johnson, Bryan J.
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NOAA Earth Syst Res Lab, Boulder, CO 80305 USAPrinceton Univ, Princeton, NJ 08540 USA
Johnson, Bryan J.
Middlebrook, Ann M.
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NOAA Earth Syst Res Lab, Boulder, CO 80305 USAPrinceton Univ, Princeton, NJ 08540 USA
Middlebrook, Ann M.
Oltmans, Samuel J.
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Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USAPrinceton Univ, Princeton, NJ 08540 USA
Oltmans, Samuel J.
Pollack, Ilana B.
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Univ Colorado, Cooperat Inst Res Environm Sci, Boulder, CO 80309 USA
NOAA Earth Syst Res Lab, Boulder, CO 80305 USAPrinceton Univ, Princeton, NJ 08540 USA
Pollack, Ilana B.
Ryerson, Tomas B.
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NOAA Earth Syst Res Lab, Boulder, CO 80305 USAPrinceton Univ, Princeton, NJ 08540 USA