Synthesis and characterization of multiferroic Pb(Zr,Ti)O3/CoFe2O4/Pb(Zr,Ti)O3 layered composite thin films by chemical solution deposition

被引：7
|
作者：
Kawabata, Yoshikatsu [1 ]
Sakamoto, Wataru [1 ]
Yoshida, Kenji [1 ]
Iijima, Takashi [2 ]
Moriya, Makoto [1 ]
Yogo, Toshinobu [1 ]
机构：
[1] Nagoya Univ, EcoTopia Sci Inst, Div Nanomat Sci, Chikusa Ku, Nagoya, Aichi 4648603, Japan
[2] Natl Inst Adv Ind Sci & Technol, Tsukuba, Ibaraki 3058569, Japan
来源：
JOURNAL OF THE CERAMIC SOCIETY OF JAPAN | 2013年 / 121卷 / 1416期
关键词：
Pb(Zr; Ti)O-3; CoFe2O4; Chemical solution deposition; Layered composite film; Electrical properties; Magnetic properties; MAGNETOELECTRIC PROPERTIES; DIELECTRIC-PROPERTIES; BIFEO3; POLARIZATION; CERAMICS; STRESS;
D O I：
10.2109/jcersj2.121.614
中图分类号：
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号：
0805 ; 080502 ;
摘要：
Multiferroic Pb(Zr,Ti)O-3/CoFe2O4/Pb(Zr,Ti)O-3 layered thin films were synthesized on Pt/TiOx/SiO2/Si substrates by chemical solution deposition using metal-organic precursor solutions. Layered composite films composed of polycrystalline perovskite Pb(Zr0.52Ti0.48)O-3 and spinel CoFe2O4 phases with no secondary phases were successfully synthesized by controlling conditions such as the coating process. The layered structure of the Pb(Zr0.52Ti0.48)O-3/CoFe2O4/Pb(Zr0.52Ti0.48)O-3 was confirmed by scanning electron microscope observations. These layered films exhibited sufficiently high insulating properties, as well as ferroelectric polarization (P)-electric field (E) and ferromagnetic magnetization (M)-magnetic field (H) hysteresis loops at room temperature. Typical ferroelectric oxide strain behavior was observed under a driving AC (alternate current) field. Furthermore, due to magnetoelectric interaction between the ferroelectric and ferromagnetic (magnetostrictive) layers, the ferroelectric properties of the films altered under an applied magnetic field (approximately 0.5 T). (C) 2013 The Ceramic Society of Japan. All rights reserved.
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收藏
页码：614 / 618
页数：5
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