Black Carbon Emissions in China from 1949 to 2050

被引:241
|
作者
Wang, Rong [1 ]
Tao, Shu [1 ]
Wang, Wentao [1 ]
Liu, Junfeng [1 ]
Shen, Huizhong [1 ]
Shen, Guofeng [1 ]
Wang, Bin [1 ]
Liu, Xiaopeng [1 ]
Li, Wei [1 ]
Huang, Ye [1 ]
Zhang, Yanyan [1 ]
Lu, Yan [1 ]
Chen, Han [1 ]
Chen, Yuanchen [1 ]
Wang, Chen [1 ]
Zhu, Dan [1 ]
Wang, Xilong [1 ]
Li, Bengang [1 ]
Liu, Wenxin [1 ]
Ma, Jianmin [2 ]
机构
[1] Peking Univ, Coll Urban & Environm Sci, Lab Earth Surface Proc, Beijing 100871, Peoples R China
[2] Environm Canada, Sci & Technol Branch, Air Qual Res Div, Toronto, ON M3H 5T4, Canada
基金
中国国家自然科学基金;
关键词
POLYCYCLIC AROMATIC-HYDROCARBONS; AEROSOL EMISSIONS; INVENTORY; ENERGY; FUTURE; RESIDUES; MATTER; STRAW;
D O I
10.1021/es3003684
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Black carbon (BC) emissions from China are of global concern. A new BC emission inventory (PKU-BC(China)) has been developed with the following improvements: (1) The emission factor database was updated; (2) a 0.1 degrees x 0.1 degrees gridded map was produced for 2007 based on county-level proxies; (3) time trends were derived for 1949-2007 and predicted for 2008-2050; and (4) the uncertainties associated with the inventory were quantified. It was estimated that 1957 Gg of BC were emitted in China in 2007, which is greater than previously reported. Residential coal combustion was the largest source, followed by residential biofuel burning, coke production, diesel vehicles, and brick kilns. By using a county-level disaggregation method, spatial bias in province level disaggregation, mainly due to uneven per capita emissions within provinces, was reduced by 42.5%. Emissions increased steadily since 1949 until leveling off in the mid 1990s, due to a series of technological advances and to socioeconomic progress. BC emissions in China in 2050 are predicted to be 920-2183 Gg/yr under various scenarios; and the industrial and transportation sectors stand to benefit the most from technological improvements.
引用
收藏
页码:7595 / 7603
页数:9
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