Oxidative carbonylation of phenol to diphenyl carbonate catalyzed by Pd dinuclear complex

被引：25
|
作者：
Ishii, H
Ueda, M
Takeuchi, K
Asai, M
机构：
[1] NIMC, JCII, Joint Res Ctr Precis Polymerizat Tsukuba, Ibaraki, Osaka 3058565, Japan
[2] Yamagata Univ, Grad Sch Engn, Yamagata 9928510, Japan
来源：
JOURNAL OF MOLECULAR CATALYSIS A-CHEMICAL | 1999年 / 144卷 / 03期
关键词：
oxidative carbonylation; diphenyl carbonate; phenol; carbon monoxide; palladium; dinuclear complex;
D O I：
10.1016/S1381-1169(99)00008-4
中图分类号：
O64 [物理化学（理论化学）、化学物理学];
学科分类号：
070304 ; 081704 ;
摘要：
Pd dinuclear complexes were investigated as catalysts for direct synthesis of diphenyl carbonate (DPC) by oxidative carbonylation of phenol using carbon monoxide and air. Pd dinuclear complexes such as Pd-2(dpm)(2)X-2 [dpm: bis(diphenylphosphino)methane, X: Cl, Br, I, OCN, SCN. N2O, N-3] were found to be novel catalysts for the oxidative carbonylation of phenol. Pd-2(dpm)(2)(OCN)(2)/Mn(TMHD)(3)/(Ph3P=)(2)NBr system was more effective than conventional Pd mononuclear catalyst. (C) 1999 Elsevier Science B.V. All rights reserved.
引用
收藏
页码：477 / 480
页数：4
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