Polaron dynamics in two-dimensional photon-echo spectroscopy of molecular rings

被引：43

作者：

Thanh Duc Huynh ^{[1
]}

Sun, Ke-Wei ^{[1
,2
]}

Gelin, Maxim ^{[3
]}

Zhao, Yang ^{[1
]}

机构：

[1] Nanyang Technol Univ, Sch Mat Sci & Engn, Singapore 639798, Singapore

[2] Hangzhou Dianzi Univ, Sch Sci, Hangzhou 310018, Zhejiang, Peoples R China

[3] Tech Univ Munich, Dept Chem, D-85747 Garching, Germany

来源：

JOURNAL OF CHEMICAL PHYSICS | 2013年 / 139卷 / 10期

基金：

新加坡国家研究基金会;

关键词：

INFRARED VIBRATIONAL ECHO; PUMP-PROBE SPECTROSCOPY; LH2 ANTENNA COMPLEXES; HARVESTING SYSTEM-II; LYING EXCITED-STATES; ELECTRONIC SPECTROSCOPY; PURPLE BACTERIA; ENERGY-TRANSFER; SUPERRADIANT EMISSION; OPTICAL SPECTROSCOPY;

D O I：

10.1063/1.4820135

中图分类号：

O64 [物理化学（理论化学）、化学物理学];

学科分类号：

070304 ; 081704 ;

摘要：

We have developed a new approach to the computation of third-order spectroscopic signals of molecular rings, by incorporating the Davydov soliton theory into the nonlinear response function formalism. The Davydov D-1 and (D) over tilde Ansatze have been employed to treat the interactions between the excitons and the primary phonons, allowing for a full description of arbitrary exciton-phonon coupling strengths. As an illustration, we have simulated a series of optical 2D spectra for two models of molecular rings. (C) 2013 AIP Publishing LLC.

引用

页数：11

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