Interrelationship of Pyrogenic Polycyclic Aromatic Hydrocarbon (PAH) Contamination in Different Environmental Media

被引:16
|
作者
Kim, Seung-Kyu [1 ,2 ]
Lee, Dong Soo [1 ]
Shim, Won Joon [3 ]
Yim, Un Hyuk [3 ]
Shin, Yong-Seung [4 ]
机构
[1] Seoul Natl Univ, Environm Planning Inst, Grad Sch Environm Studies, Seoul 151742, South Korea
[2] Seoul Natl Univ, Sch Earth & Environm Sci BK 21, Seoul 151742, South Korea
[3] Korea Ocean Res & Dev Inst, Oil & POPs Res Grp, Jangmok Myon 656834, Geoje Shi, South Korea
[4] Korea Environm Inst, Environm Policy Div, Seoul 122706, South Korea
关键词
PAHs; fugacity ratio; multi-media fate; partitioning equilibrium; black carbon; PERSISTENT ORGANIC POLLUTANTS; MASS-BALANCE MODELS; BLACK CARBON; POLYCHLORINATED-BIPHENYLS; SIZE DISTRIBUTIONS; MULTIMEDIA MODEL; DRY DEPOSITION; LAW CONSTANTS; URBAN; FATE;
D O I
10.3390/s91209582
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Interrelationships between pyrogenic polycyclic aromatic hydrocarbons (PAHs) were assessed in air, soil, water, sediment, and tree leaves by using multi-media monitoring data. Concurrent concentration measurements were taken bimonthly for a year for the multi-media at urban and suburban sites. PAH level correlations between air and other media were observed at the urban site but were less clear at the suburban site. Considering a closer PAHs distribution/fate characteristics to soil than suspended solids, contamination in sediment seemed to be governed primarily by that in soil. The partitioning of PAHs in waters could be better accounted for by sorption onto black carbon and dissolved organic carbon.
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页码:9582 / 9602
页数:21
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