Distribution, sources and health risk assessment of mercury in kindergarten dust

被引:48
|
作者
Sun, Guangyi [1 ,3 ,4 ]
Li, Zhonggen [2 ]
Bi, Xiangyang [1 ]
Chen, Yupeng [2 ]
Lu, Shuangfang [4 ]
Yuan, Xin [5 ]
机构
[1] China Univ Geosci, State Key Lab Biogeol & Environm Geol, Wuhan 430074, Peoples R China
[2] Chinese Acad Sci, Inst Geochem, State Key Lab Environm Geochem, Guiyang 550002, Peoples R China
[3] Hei Longjiang Inst Geol Survey, Harbin 150036, Peoples R China
[4] Northeast Petr Univ, Fac Earth Sci, Daqing 163318, Peoples R China
[5] LEU, Dept Barracks Management & Environm Engn, Chongqing 401131, Peoples R China
基金
美国国家科学基金会;
关键词
Mercury; Methylmercury; Kindergarten dust; Risk assessment; Wuhan city; ATMOSPHERIC MERCURY; TRACE-ELEMENTS; EMISSIONS; EXPOSURE; CHINA; CONTAMINATION; CHILDREN; GUIZHOU; TOPSOIL; SOIL;
D O I
10.1016/j.atmosenv.2013.03.017
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
Mercury (Hg) contamination in urban area is a hot issue in environmental research. In this study, the distribution, sources and health risk of Hg in dust from 69 kindergartens in Wuhan, China, were investigated. In comparison with most other cities, the concentrations of total mercury (THg) and methylmercury (MeHg) were significantly elevated, ranging from 0.15 to 10.59 mg kg(-1) and from 0.64 to 3.88 mu g kg(-1), respectively. Among the five different urban areas, the educational area had the highest concentrations of THg and MeHg. The GIS mapping was used to identify the hot-spot areas and assess the potential pollution sources of Hg. The emissions of coal-power plants and coking plants were the main sources of THg in the dust, whereas the contributions of municipal solid waste (MSW) landfills and iron and steel smelting related industries were not significant. However, the emission of MSW landfills was considered to be an important source of MeHg in the studied area. The result of health risk assessment indicated that there was a high adverse health effect of the kindergarten dust in terms of Hg contamination on the children living in the educational area (Hazard index (HI) = 6.89). (C) 2013 Elsevier Ltd. All rights reserved.
引用
收藏
页码:169 / 176
页数:8
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