One-step nanocasting synthesis of sulfur and nitrogen co-doped ordered mesoporous carbons as efficient electrocatalysts for oxygen reduction

被引：13

作者：

Song, Xiaozeng ^{[1
]}

Ren, Hongxin ^{[1
]}

Ding, Junjie ^{[1
]}

Wang, Chenfei ^{[1
]}

Yin, Xin ^{[1
]}

Wang, Haiwen ^{[1
]}

机构：

[1] E China Univ Sci & Technol, Sch Chem & Mol Engn, Shanghai 200237, Peoples R China

来源：

MATERIALS LETTERS | 2015年 / 159卷

基金：

中国国家自然科学基金;

关键词：

Carbon materials; Porous materials; Oxygen reduction reaction; Fuel cell; METAL-FREE ELECTROCATALYSTS; CATALYSTS; GRAPHENE; BORON;

D O I：

10.1016/j.matlet.2015.06.112

中图分类号：

T [工业技术];

学科分类号：

08 ;

摘要：

Ordered mesoporous carbon co-doped with sulfur and nitrogen (SN-OMC) is synthesized via one-step nanocasting route. Diphenylthiocarbazone is used as a single precursor for carbon, sulfur and nitrogen in the preparation of SN-OMCs. These catalysts are subjected to the physicochemical characterization and electrochemical evaluation toward the oxygen reduction reaction (ORR) in an alkaline electrolyte. SN-OMC obtained at 900 degrees C exhibits a high electrocatalytic activity for ORR and the impressive durability and methanol-tolerance. The synergistic effect of nitrogen and sulfur in mesoporous carbon walls may contribute to high oxygen electroreduction performance of SN-OMC. (C) 2015 Elsevier B.V. All rights reserved.

引用

页码：280 / 283

页数：4

共 50 条

[1] One-step nanocasting synthesis of nitrogen and phosphorus dual heteroatom doped ordered mesoporous carbons for supercapacitor application
Feng, Jian
Song, Weiming
Sun, Li
Xu, Liyang
RSC ADVANCES, 2016, 6 (111): : 110337 - 110343
[2] Nitrogen and Sulfur Co-doped Mesoporous Carbon Materials as Highly Efficient Electrocatalysts for Oxygen Reduction Reaction
Shi, Jingjing
Zhou, Xuejun
Xu, Pan
Qiao, Jinli
Chen, Zhongwei
Liu, Yuyu
ELECTROCHIMICA ACTA, 2014, 145 : 259 - 269
[3] Nitrogen and sulfur co-doped mesoporous hollow carbon microspheres for highly efficient oxygen reduction electrocatalysts
Zhao, Hui
Zhu, Yun-Pei
Ge, Li
Yuan, Zhong-Yong
INTERNATIONAL JOURNAL OF HYDROGEN ENERGY, 2017, 42 (30) : 19010 - 19018
[4] In-situ synthesis of heteroatom co-doped mesoporous dominated carbons as efficient electrocatalysts for oxygen reduction reaction
Liu, Jianting
Wei, Liling
Wang, Huiqiang
Lan, Gongjia
Yang, Haijun
Shen, Jianquan
ELECTROCHIMICA ACTA, 2020, 364
[5] One-pot synthesis of boron-doped ordered mesoporous carbons as efficient electrocatalysts for the oxygen reduction reaction
Su, Jianmin
Cao, Xuecheng
Wu, Jiao
Jin, Chao
Tian, Jing-Hua
Yang, Ruizhi
RSC ADVANCES, 2016, 6 (29) : 24728 - 24737
[6] One-Step Production of Sulfur and Nitrogen Co-doped Graphitic Carbon for Oxygen Reduction: Activation Effect of Oxidized Sulfur and Nitrogen
Wang, Jing
Xu, Zheng
Gong, Yutong
Han, Chuanlong
Li, Haoran
Wang, Yong
CHEMCATCHEM, 2014, 6 (05) : 1204 - 1209
[7] Facile One-step Synthesis of Ordered Mesoporous Carbons Doped with Nickel Particles
Li, Peng
Song, Yan
Geng, Yu
Zhong, Ming
Guo, Quangui
Shi, Jingli
Liu, Lang
INTERNATIONAL JOURNAL OF ELECTROCHEMICAL SCIENCE, 2012, 7 (05): : 4039 - 4046
[8] One-step Nanocasting Synthesis of Ordered Mesoporous Carbon with Graphitic Frameworks
Wang, Yangang
Wang, Fei
Chen, Yuting
Li, Bo
Zhang, Chengli
Cui, Lifeng
Kang, Shifei
Li, Xi
INTERNATIONAL JOURNAL OF ELECTROCHEMICAL SCIENCE, 2013, 8 (06): : 7868 - 7874
[9] One-pot synthesis of nitrogen and sulfur co-doped graphene as efficient metal-free electrocatalysts for the oxygen reduction reaction
Wang, Xin
Wang, Jie
Wang, Deli
Dou, Shuo
Ma, Zhaoling
Wu, Jianghong
Tao, Li
Shen, Anli
Ouyang, Canbin
Liu, Qiuhong
Wang, Shuangyin
CHEMICAL COMMUNICATIONS, 2014, 50 (37) : 4839 - 4842
[10] Hierarchical porous iron and nitrogen co-doped carbons as efficient oxygen reduction electrocatalysts in neutral media
Su, Yunhe
Jiang, Hongliang
Zhu, Yihua
Zou, Wenjian
Yang, Xiaoling
Chen, Jianding
Li, Chunzhong
JOURNAL OF POWER SOURCES, 2014, 265 : 246 - 253

← 1 2 3 4 5 →