Cooperative sequential adsorption of k-mers on heterogeneous substrates

被引:2
|
作者
Zuppa, C
Ciacera, M
Zgrablich, G [1 ]
机构
[1] Univ Nacl San Luis, Lab Ciencias Superficies & Medios Porosos, RA-5700 San Luis, Argentina
[2] Univ Nacl San Luis, Ctr Latinoamer Estudios Ilya Prigogine, RA-5700 San Luis, Argentina
[3] Univ Nacl San Luis, Dept Matemat, RA-5700 San Luis, Argentina
关键词
D O I
10.1021/la981338y
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
The cooperative sequential adsorption of dimers and trimers on heterogeneous substrates with random and patchwise (chessboard and strip) topographies is studied by Monte Carlo simulation. Strong influence of the topography is found on the adsorption kinetics, measured through the dependence of the sticking coefficient with the surface coverage, and the jamming coverage. In particular, an unexpected behavior of the jamming coverage is found for dimers and trimers on a random topography, which, unlike the case of dimers in one dimension, differs from that corresponding to a homogeneous surface.
引用
收藏
页码:5984 / 5989
页数:6
相关论文
共 50 条
  • [1] Adsorption of linear k-mers on heterogeneous surfaces with simple topographies
    Ramirez-Pastor, AJ
    Riccardo, JL
    Pereyra, V
    [J]. LANGMUIR, 2000, 16 (02) : 682 - 689
  • [2] Cooperative sequential adsorption on heterogeneous substrates
    Ciacera, M
    Zgrablich, G
    [J]. SURFACES, VACUUM, AND THEIR APPLICATIONS, 1996, (378): : 593 - 596
  • [3] Random sequential adsorption of k-mers on a square lattice: The large k regime
    Bonnier, B
    [J]. PHYSICAL REVIEW E, 1996, 54 (01): : 974 - 976
  • [4] Random sequential adsorption and diffusion of dimers and k-mers on a square lattice
    Fusco, C
    Gallo, P
    Petri, A
    Rovere, M
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2001, 114 (17): : 7563 - 7569
  • [5] RANDOM SEQUENTIAL ADSORPTION OF DIFFERENT-SIZED K-MERS ON A LINE
    RODGERS, GJ
    [J]. PHYSICAL REVIEW A, 1992, 45 (06): : 3432 - 3434
  • [6] Random sequential adsorption of partially oriented linear k-mers on a square lattice
    Lebovka, Nikolai I.
    Karmazina, Natalia N.
    Tarasevich, Yuri Yu.
    Laptev, Valeri V.
    [J]. PHYSICAL REVIEW E, 2011, 84 (06):
  • [7] Monte Carlo simulation of the percolation process caused by the random sequential adsorption of k-mers on heterogeneous triangular lattices
    Quintana, M
    Kornhauser, I
    López, R
    Ramirez-Pastor, AJ
    Zgrablich, G
    [J]. PHYSICA A-STATISTICAL MECHANICS AND ITS APPLICATIONS, 2006, 361 (01) : 195 - 208
  • [8] Cooperative sequential adsorption processes on heterogeneous substrates
    Stacchiola, DJ
    Ciacera, M
    Zuppa, C
    Eggarter, TP
    Zgrablich, G
    [J]. JOURNAL OF CHEMICAL PHYSICS, 1998, 108 (04): : 1730 - 1739
  • [9] Irreversible sequential adsorption of k-mers with diffusional relaxation on a one-dimensional lattice
    Lee, JW
    Hong, BH
    [J]. JOURNAL OF CHEMICAL PHYSICS, 2003, 119 (01): : 533 - 537
  • [10] Impact of defects on percolation in random sequential adsorption of linear k-mers on square lattices
    Astrakhan State University, Astrakhan
    414056, Russia
    不详
    414056, Russia
    不详
    03142, Ukraine
    [J]. Phys. Rev. E Stat. Nonlinear Soft Matter Phys., 1