UV-light -assisted ethanol sensing characteristics of g-C3N4/ZnO composites at room temperature

被引:49
|
作者
Zhai, Jiali [1 ]
Wang, Tao [1 ]
Wang, Chuang [1 ]
Liu, Dechen [1 ]
机构
[1] Jilin Police Coll, Dept Forens Sci, Engn Res Ctr Forens Sci, Changchun 130102, Jilin, Peoples R China
基金
中国国家自然科学基金;
关键词
UV-light-assisted; Composites; g-C3N4/ZnO; Room temperature sensor; GRAPHITIC CARBON NITRIDE; VISIBLE-LIGHT; PHOTOCATALYTIC ACTIVITY; GAS SENSORS; PHASE C3N4; THIN-FILMS;
D O I
10.1016/j.apsusc.2018.02.026
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
A highly efficient UV-light-assisted room temperature sensor based on g-C3N4/ZnO composites were prepared by an in situ precipitation method. The thermostability, composition, structure, and morphology properties of the as-prepared g-C3N4/ZnO composites were characterized by TGA, XRD, FT-IR, TEM, and XPS, respectively. And then, we studied the ethanol (C2H5OH) sensing performance of the g-C3N4/ZnO composites at the room temperature. Compared with pure ZnO and g-C3N4, the gas sensing activity of g-C3N4/ZnO composites was greatly improved at room temperature, for example, the g-C3N4/ZnO-8% composites showed an obvious response of 121-40 ppm C2H5OH at room temperature, which was 60 times higher than the pure ZnO based on the sensors under the same condition. The great enhancement of the C2H5OH sensing properties of composites can be understood by the efficient separation of photogenerated charge carriers of g-C3N4/ZnO heterogeneous and the UV-light catalytic effect. Finally, a possible mechanism for the gas sensing activity was proposed. (C) 2018 Elsevier B.V. All rights reserved.
引用
收藏
页码:317 / 323
页数:7
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