Active glassy dynamics is unaffected by the microscopic details of self-propulsion

被引:8
|
作者
Debets, Vincent E. [1 ,2 ]
Janssen, Liesbeth M. C. [1 ,2 ]
机构
[1] Eindhoven Univ Technol, Dept Appl Phys, POB 513, NL-5600 MB Eindhoven, Netherlands
[2] Eindhoven Univ Technol, Inst Complex Mol Syst, POB 513, NL-5600 MB Eindhoven, Netherlands
来源
JOURNAL OF CHEMICAL PHYSICS | 2022年 / 157卷 / 22期
基金
荷兰研究理事会;
关键词
MODE-COUPLING THEORY; TRANSITION; PARTICLES; CELL;
D O I
10.1063/5.0127569
中图分类号
O64 [物理化学(理论化学)、化学物理学];
学科分类号
070304 ; 081704 ;
摘要
Recent years have seen a rapid increase of interest in dense active materials, which, in the disordered state, share striking similarities with the conventional passive glass-forming matter. For such passive glassy materials, it is well established (at least in three dimensions) that the details of the microscopic dynamics, e.g., Newtonian or Brownian, do not influence the long-time glassy behavior. Here, we investigate whether this still holds true in the non-equilibrium active case by considering two simple and widely used active particle models, i.e., active Ornstein-Uhlenbeck particles (AOUPs) and active Brownian particles (ABPs). In particular, we seek to gain more insight into the role of the self-propulsion mechanism on the glassy dynamics by deriving a mode-coupling theory (MCT) for thermal AOUPs, which can be directly compared to a recently developed MCT for ABPs. Both theories explicitly take into account the active degrees of freedom. We solve the AOUP- and ABP-MCT equations in two dimensions and demonstrate that both models give almost identical results for the intermediate scattering function over a large variety of control parameters (packing fractions, active speeds, and persistence times). We also confirm this theoretical equivalence between the different self-propulsion mechanisms numerically via simulations of a polydisperse mixture of active quasi-hard spheres, thereby establishing that, at least for these model systems, the microscopic details of self-propulsion do not alter the active glassy behavior. Published under an exclusive license by AIP Publishing.
引用
收藏
页数:11
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