Radiation force exerted on nanometer size non-resonant Kerr particle by a tightly focused Gaussian beam

We calculate the radiation force that is exerted by a focused continuous-wave Gaussian beam of wavelength), on a non-absorbing nonlinear particle of radius a <= 50 lambda/pi. The refractive index of the mechanically-rigid particle is proportional to the incident intensity according to the electro-optic Kerr effect. The force consists of two components representing the contributions of the electromagnetic field gradient and the light scattered by the Kerr particle. The focused intensity distribution is determined using expressions for the six electromagnetic components that are corrected to the fifth order in the numerical aperture (NA) of the focusing objective lens. We found that for particles with a < lambda/21.28, the trapping force is dominated by the gradient force and the axial trapping force is symmetric about the geometrical focus. The two contributions are comparable with larger particles and the axial trapping force becomes asymmetric with its zero location displaced away from the focus and towards the beam propagation direction. We study the trapping force behavior versus incident beam power, NA, lambda, and relative refractive index between the surrounding liquid and the particle. We also examine the confinement of a Kerr particle that exhibits Brownian motion in a focused beam. Numerical results show that the Kerr effect increases the trapping force strength and significantly improves the confinement of Brownian particles. (c) 2006 Elsevier B.V. All rights reserved.