Development, dilemma and potential strategies for the application of nanocatalysts in wastewater catalytic ozonation: A review

被引:40
|
作者
Jin, Xiaoguang [1 ,2 ,3 ]
Wu, Changyong [1 ,3 ]
Fu, Liya [1 ,3 ]
Tian, Xiangmiao [1 ,2 ,3 ]
Wang, Panxin [1 ,3 ]
Zhou, Yuexi [1 ,3 ]
Zuo, Jiane [2 ]
机构
[1] Chinese Res Inst Environm Sci, State Key Lab Environm Criteria & Risk Assessment, Beijing 100012, Peoples R China
[2] Tsinghua Univ, Sch Environm, Beijing 100084, Peoples R China
[3] Chinese Res Inst Environm Sci, Res Ctr Environm Pollut Control Engn Technol, Beijing 100012, Peoples R China
来源
关键词
Catalytic ozonation; Nanocatalyst limitation; Membrane; Supported nanocatalysts; Magnetic nanocatalysts; MULTIWALLED CARBON NANOTUBES; REDUCED GRAPHENE OXIDE; NANO-PERFLUOROOCTYL ALUMINA; NITROGEN-DOPED GRAPHENE; MONTE-CARLO-SIMULATION; HIGH-SURFACE-AREA; TERT-BUTYL ETHER; ORGANIC CONTAMINANTS; ENHANCED OZONATION; AQUEOUS-SOLUTIONS;
D O I
10.1016/j.jes.2021.09.041
中图分类号
X [环境科学、安全科学];
学科分类号
08 ; 0830 ;
摘要
With the continuous development of nanomaterials in recent years, the application of nanocatalysts in catalytic ozone oxidation has attracted more and more researchers' at-tention due to their excellent catalytic properties. In this review, we systematically sum-marized the current research status of nanocatalysts mainly involving material categories, mechanisms and catalytic efficiency. Based on summary and analysis, we found most of the reported nanocatalysts were in the stage of laboratory research, which was caused by the nanocatalysts defects such as easy aggregation, difficult separation, and easy leakage. These defects might result in severe resource waste, economic loss and potentially adverse effects imposed on the ecosystem and human health. Aiming at solving these defects, we further analyzed the reasons and the existing reports, and revealed that coupling nano-catalyst and membrane, supported nanocatalysts and magnetic nanocatalysts had promising po-tential in solving these problems and promoting the actual application of nanocatalysts in wastewater treatment. Furthermore, the advantages, shortages and our perspectives of these methods are summarized and discussed. (c) 2022 The Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences. Published by Elsevier B.V.
引用
收藏
页码:330 / 349
页数:20
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