Precise Control of Single-Crystal Perovskite Nanolasers

被引:5
|
作者
Zhuge, Minghua [1 ,2 ]
Yin, Jun [1 ,2 ]
Liu, Yilin [1 ,2 ]
Wang, Yuhan [1 ,2 ]
Li, Ziyu [1 ,2 ]
Xiao, Shumin [1 ,2 ,3 ,4 ]
Yu, Shaohua [3 ]
Song, Qinghai [1 ,2 ,3 ,4 ]
机构
[1] Harbin Inst Technol, Minist Ind & Informat Technol, Key Lab Micronano Optoelect Informat Syst, Shenzhen 518055, Peoples R China
[2] Guangdong Prov Key Lab Semicond, Shenzhen 518055, Peoples R China
[3] Pengcheng Lab, Shenzhen 518055, Peoples R China
[4] Shanxi Univ, Collaborat Innovat Ctr Extreme Opt, Taiyuan 030006, Shanxi, Peoples R China
基金
中国博士后科学基金; 中国国家自然科学基金;
关键词
chirality; exceptional points; far-field emission direction; perovskites; precise control; LASERS;
D O I
10.1002/adma.202300344
中图分类号
O6 [化学];
学科分类号
0703 ;
摘要
Efficient control of integrated light sources is crucial to advancing practical applications of nanophotonics. Despite the success of microlasers, their sophisticated nanostructures are not applicable in nanolasers. The situation for bottom-up-synthesized nanolasers becomes more challenging due to the constraints of fixed cavity shapes and fragile material stability. Here, the physics of exceptional points (EPs) is employed, and a strategy is demonstrated to precisely tune the lasing actions in lead halide perovskite nanorods. By placing a nanoparticle to the boundary of a square nanocavity, it is shown that EPs regularly and controllably emerge as a function of the nanoparticle position. Consequently, both the internal lasing actions and their far-field radiation can be completely reversed with a tiny displacement of <100 nm. The new strategy for controlling lasing actions in nanocavities is confirmed with numerical simulations and lasing experiments. This research can also bring new avenues for ultrasensitive position sensing.
引用
收藏
页数:8
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