Climatology and landscape determinants of AOD, SO2 and NO2 over Indo-Gangetic Plain

Indo-Gangetic Plains (IGP) experiences high loading of particulate and gaseous pollutants all year around and is considered to be the most polluted regions of India. Understanding the effect of landscape determinants on air pollution in IGP regions is crucial to make its environment sustainable. We examined satellite retrievals of OMI NO2 and SO2, and MODIS AOD to analyse the long-term trend, spatio-seasonal pattern and dynamics of aerosols, NO2 and SO2 over three IGP regions, namely Upper Indo-Gangetic plain (UIGP), Middle Indo-Gangetic plain (MIGP) and Lower Indo-Gangetic plain (LIGP) over the period 2005-2019. IGP experienced an overall increment in AOD (R2 = 0.63) and SO2 (R2 = 0.67) values, with LIGP (AOD, R2 = 0.8 & SO2, R2 = 0.8) experiencing the largest rate of enhancement. The levels of NO2 (R2 = 0.2) experienced a decrement after 2012 (owing to implementation of vehicle emission policy) except in MIGP, with UIGP (R2 = 0.23) exhibiting the largest rate of decrement. Seasonal heterogeneity in the nature of sources was observed over IGP regions. AOD (0.61 +/- 0.1) and NO2 value (3.82 +/- 0.98 x 1015 molecules/cm2) were found highest during post-monsoon in UIGP owing to crop residue burning activity. The value of NO2 (3.8 +/- 1.4 x 1015 molecules/cm2) in MIGP was found highest during pre-monsoon due to high consumption of coal in power plants for summer cooling demand. The highest SO2 level (0.09 +/- 0.06 DU) was observed during post-monsoon in UIGP, as a large number of brick kilns are fired during this period. Correlations among landscape determinants and pollutants revealed that topography is the dominant variable that affect the spatial pattern of AOD compared to vegetation and land use. Lower elevation tends to have high AOD values compared to higher elevation. Vegetation-AOD relationship showed an inverse association in IGP regions and is influenced by factors such as seasonal meteorology and size of the airborne particles. Vegetation possesses positive relationship with SO2 and NO2, implying no pollution abatement effect on SO2 and NO2 pollutants. Built-up change has deteriorating effect as well as quenching effect on pollutants. Increase in built terrain have deteriorated the air quality in UIGP whereas it favored in suppressing the aerosol level in LIGP.