Preparation of exposed (001) facets TiO2/Ti3C2 MXene and performance of near infrared light photodegradation

被引:10
|
作者
Wang, Yong [1 ]
Tan, Guoqiang [1 ]
Feng, Shuaijun [1 ]
Liu, Yun [2 ]
Liu, Wenlong [2 ]
Xia, Ao [1 ]
Ren, Huijun [3 ]
Lv, Long [4 ]
机构
[1] Shaanxi Univ Sci Technol, Sch Mat Sci & Engn, Shaanxi Key Lab Green Preparat & Functionalizat I, Xian 710021, Peoples R China
[2] Shaanxi Univ Sci Technol, Sch Elect Informat & Artificial Intelligence, Xian 710021, Peoples R China
[3] Shaanxi Univ Sci Technol, Sch Arts & Sci, Xian 710021, Peoples R China
[4] China Acad Space Technol, Xian 710100, Peoples R China
基金
中国国家自然科学基金;
关键词
(001)TiO2/Ti3C2 MXene; Local surface plasmon resonance; Near infrared light degradation; Tetracycline; PHOTOCATALYTIC DEGRADATION; TI3C2; ADSORPTION;
D O I
10.1016/j.ceramint.2022.10.157
中图分类号
TQ174 [陶瓷工业]; TB3 [工程材料学];
学科分类号
0805 ; 080502 ;
摘要
The (001)TiO2/Ti3C2 MXene heterojunction photocatalyst was prepared with the hydrothermal oxidation method by using the two-dimensional Ti3C2 MXene as the substrate. The formation of TiO2 surface hetero-junctions, Schottky junctions at the interface between (001) facets TiO2 and Ti3C2 MXene, and the local surface plasmon resonance effect of plasma Ti3C2 MXene combine together to promote the effective separation of electrons and holes after photoexcitation. After 150 min of near infrared light irradiation and sunlight irradiation, the degradation rates of tetracycline by (001)TiO2/Ti3C2 MXene photocatalyst are 28.63% and 52.74%, respectively, with near infrared light and full spectrum degradation characteristics. Our work is expected to provide a valuable reference for the design of MXene based full spectrum photocatalysts.
引用
收藏
页码:7258 / 7265
页数:8
相关论文
共 50 条
  • [1] Preparation and Visible Light Photocatalytic Performance of BiOBr/Ti3C2 Composite Photocatalyst with Highly Exposed (001) Facets
    Li Zhifeng
    Tan Jie
    Yang Xiaofei
    Lin Zuhong
    Huan Zhenglai
    Zhang Tingting
    JOURNAL OF INORGANIC MATERIALS, 2020, 35 (11) : 1247 - 1254
  • [2] Ti3C2 MXene derived (001)TiO2/Ti3C2 heterojunctions for enhanced visible-light photocatalytic degradation of tetracycline
    Qiang, Wei
    Qu, Xiao
    Chen, Chuntao
    Zhang, Lei
    Sun, Dongping
    MATERIALS TODAY COMMUNICATIONS, 2022, 33
  • [3] Preparation of Two Dimensional TiO2/Ti3C2 Photocatalyst by Solvothermal Oxidation of Few-Layered Ti3C2 MXene
    Yan Kang
    Guan Yun-Feng
    Cong Ye
    Xu Tian-Xiang
    Zhu Hui
    Li Xuan-Ke
    CHINESE JOURNAL OF INORGANIC CHEMISTRY, 2019, 35 (07) : 1203 - 1211
  • [4] Ti3C2 MXene nanosheet/TiO2 composites for efficient visible light photocatalytic activity
    Chen, Long
    Ye, Xiaoyun
    Chen, Song
    Ma, Lian
    Wang, Zhaopeng
    Wang, Qianting
    Hua, Nengbin
    Xiao, Xueqing
    Cai, Shuguang
    Liu, Xuehua
    CERAMICS INTERNATIONAL, 2020, 46 (16) : 25895 - 25904
  • [5] Preparation and Photocatalytic Performance of Ti3C2/TiO2/CuO Ternary Nanocomposites
    Lu, Yang
    Yao, Meihuan
    Zhou, Aiguo
    Hu, Qianku
    Wang, Libo
    JOURNAL OF NANOMATERIALS, 2017, 2017
  • [6] Preparation of C–TiO2 photocatalyst with Ti3C2 MXene as precursor by molten salt method and its hydrogen production performance
    Xinxin Jin
    Minmin Yan
    Yanli Zhuang
    Limin Dong
    Haixia Wang
    Hao Niu
    Shaokai Hou
    Lianwei Shan
    Xiao Li
    Fengming Zhang
    Journal of Materials Science, 2023, 58 : 302 - 316
  • [7] Composites of TiO2 Nanoparticles Deposited on Ti3C2 MXene Nanosheets with Enhanced Electrochemical Performance
    Zhu, JianFeng
    Tang, Yi
    Yang, ChenHui
    Wang, Fen
    Cao, MinJuan
    JOURNAL OF THE ELECTROCHEMICAL SOCIETY, 2016, 163 (05) : A785 - A791
  • [8] Hybrids of Two-Dimensional Ti3C2 and TiO2 Exposing {001} Facets toward Enhanced Photocatalytic Activity
    Peng, Chao
    Yang, Xianfeng
    Li, Yuhang
    Yu, Hao
    Wang, Hongjuan
    Peng, Feng
    ACS APPLIED MATERIALS & INTERFACES, 2016, 8 (09) : 6051 - 6060
  • [9] Fabrication and photocatalytic performance of highly active exposed facets ZnO hexagonal cap/Ti3C2 MXene composites
    Zeng, Bin
    Ning, Xutao
    Li, Linfang
    JOURNAL OF ALLOYS AND COMPOUNDS, 2023, 963
  • [10] MXene-derived C-doped TiO2/Ti3C2 heterojunction as a high-performance visible-light photocatalyst
    Kai Chen
    Kang Yan
    Qun Xie
    Hui Zhu
    Xuanke Li
    Zhijun Dong
    Guanming Yuan
    Jiang Zhang
    Ye Cong
    Research on Chemical Intermediates, 2022, 48 : 4443 - 4458