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Synergistic effect of non-thermal plasma and CH4 addition on turbulent NH3/air premixed flames in a swirl combustor
被引:7
|作者:
Kim, Gyeong Taek
[1
,2
]
Park, Jeong
[3
]
Chung, Suk Ho
[4
]
Yoo, Chun Sang
[1
]
机构:
[1] Ulsan Natl Inst Sci & Technol, Dept Mech Engn, Ulsan 44919, South Korea
[2] POSCO HOLDINGS, Hydrogen & Low Carbon Energy R&D Lab, Pohang 37673, South Korea
[3] Pukyong Natl Univ, Dept Mech Engn, Busan 48547, South Korea
[4] King Abdullah Univ Sci & Technol, Clean Combust Res Ctr, Thuwal, Saudi Arabia
基金:
新加坡国家研究基金会;
关键词:
Swirl-stabilizedNH3/Air premixed flame;
CH4;
addition;
Non-thermal plasma (NTP);
Streamer;
NOx/CO emissions;
LAMINAR BURNING VELOCITY;
AMMONIA;
NOX;
EMISSIONS;
KINETICS;
ENERGY;
IONS;
FLOW;
D O I:
10.1016/j.ijhydene.2023.08.213
中图分类号:
O64 [物理化学(理论化学)、化学物理学];
学科分类号:
070304 ;
081704 ;
摘要:
The synergistic effect of non-thermal plasma (NTP) induced by a dielectric barrier discharge (DBD) and CH4 addition on turbulent swirl-stabilized NH3/air premixed flames in a laboratory-scale gas turbine combustor is experimentally investigated by varying the mixture equivalence ratio, phi, the mixt velocity, U-0, and the mole fraction of CH4 in the fuel, X-f,X-CH4. It is found that the streamer intensity is significantly increased by adding CH4 to NH3/air flames compared with that by adding H-2. This is because positive ions generated by CH4 addition play a critical role in generating streamers. Such streamers intensified by CH4 addition enhance the ammonia combustion more together with CH4, and hence, the lean blowout (LBO) limits of NH3/CH4/air flames are significantly extended compared with those without applying NTP. The maximum streamer intensity is found to be linearly proportional to phi, X-f,X-CH4 in wide ranges of phi, X-f,X-CH4, and U-0. NTP is also found to significantly reduce the amount of NOx and CO emissions simultaneously. All of the results suggest that NTP can be used more effectively with CH4 addition to stabilize turbulent premixed NH3/air flames and reduce NOx/CO emissions, which is attributed to their synergistic effect on the ammonia combustion.
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页码:521 / 532
页数:12
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