IN-SITU OBSERVATIONS;
FRACTIONAL RELEASE FACTORS;
CHEMICAL LAGRANGIAN MODEL;
STRATOSPHERIC WATER-VAPOR;
CONVECTIVE-TRANSPORT;
EFFICIENT TRANSPORT;
UPPER TROPOSPHERE;
TROPOPAUSE LAYER;
AGE SPECTRA;
MEAN AGES;
D O I:
10.5194/acp-24-317-2024
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
During the Asian monsoon season, greenhouse gases and pollution emitted near the ground are rapidly uplifted by convection up to an altitude of similar to 13 km, with slower ascent and mixing with the stratospheric background above. Here, we address the robustness of the representation of these transport processes in different reanalysis data sets using ERA5, ERA-Interim and ERA5 1 circle x 1 circle . This transport assessment includes the mean age of air from global three-dimensional simulations by the Lagrangian transport model CLaMS (Chemical Lagrangian Model of the Stratosphere), as well as different trajectory-based transport times and associated ascent rates compared with observation-based age of air and ascent rates of long-lived trace gases from airborne measurements during the Asian summer monsoon 2017 in Nepal.Our findings confirm that the ERA5 reanalysis yields a better representation of convection than ERA-Interim, resulting in different transport times and air mass origins at the Earth's surface. In the Asian monsoon region above 430 K, the mean age of air driven by ERA-Interim is too young, whereas the mean age of air from ERA5 1 circle x 1 circle is too old but somewhat closer to the observations. The mean effective ascent rates derived from ERA5 and ERA5 1 circle x 1 circle back trajectories are in good agreement with the observation-based mean ascent rates, unlike ERA-Interim, which is much faster above 430 K. Although a reliable CO 2 reconstruction is a challenge for model simulations, we show that, up to 410 K, the CO 2 reconstruction using ERA5 agrees best with high-resolution in situ aircraft CO 2 measurements, indicating a better representation of Asian monsoon transport in the newest ECMWF reanalysis product, ERA5.