N/S co-doped carbon nanosheets derived from sugarcane processing by-products for flexible solid-state supercapacitors

被引:13
|
作者
Shi, Fangfang [1 ]
Zhang, Zhengchu [1 ]
Xu, Yongjie [1 ]
Yang, Chao [1 ]
Qiu, Jianhui [2 ]
Liao, Jiachi [3 ]
Zang, Limin [1 ]
机构
[1] Guilin Univ Technol, Guangxi Coll & Univ Key Lab Nat & Biomed Polymer M, Coll Mat Sci & Engn, Guilin 541004, Peoples R China
[2] Akita Prefectural Univ, Fac Syst Sci & Technol, Dept Machine Intelligence & Syst Engn, Yurihonjo 0150055, Japan
[3] Northwestern Polytech Univ, Queen Mary Univ London, Engn Sch, Xian 710072, Peoples R China
基金
中国国家自然科学基金;
关键词
Supercapacitor; Carbonization; Biomass -derived carbon; Sulfonated potassium fulvic acid; ANODE MATERIAL; NITROGEN; GRAPHENE; CARBONIZATION; COMPOSITES; OXIDE;
D O I
10.1016/j.jelechem.2023.117217
中图分类号
O65 [分析化学];
学科分类号
070302 ; 081704 ;
摘要
Developing sustainable carbon materials from biomass for supercapacitors is a promising solution to alleviate energy and environmental pressures. In this paper, novel N/S co-doped carbon nanosheets derived from sug-arcane processing by-products are proposed. Flexible and binder-free electrodes based on carbon felt and sul-fonated potassium fulvic acid were prepared by a simple impregnation-carbonization method. The maximum areal specific capacitance, power density and energy density of the symmetric supercapacitor are 409.9 mF cm-2 (1 mA cm-2), 0.92 mW cm-2 and 184.5 mu Wh cm-2, respectively. The operating voltage of the device increases to 1.8 V by using LiCl electrolyte. After 10,000 cycles, the capacitance remains 90 % of its initial value. Besides, the device possesses good flexibility, which can be bent at different angles and has a capacitance retention of 92.3 % after 5000 bending cycles. The supercapacitor is of great significance for the recovery of crop processing by-products to prepare flexible electronic devices.
引用
收藏
页数:9
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