Hyperuniformity of maximally random jammed packings of hyperspheres across spatial dimensions

被引:4
|
作者
Maher, Charles Emmett [1 ]
Jiao, Yang [2 ,3 ]
Torquato, Salvatore [1 ,4 ,5 ,6 ]
机构
[1] Princeton Univ, Dept Chem, Princeton, NJ 08544 USA
[2] Arizona State Univ, Mat Sci & Engn, Tempe, AZ 85287 USA
[3] Arizona State Univ, Dept Phys, Tempe, AZ 85287 USA
[4] Princeton Univ, Dept Phys, Princeton, NJ 08544 USA
[5] Princeton Univ, Princeton Mat Inst, Princeton, NJ 08544 USA
[6] Princeton Univ, Program Appl & Computat Math, Princeton, NJ 08544 USA
基金
美国国家科学基金会;
关键词
HARD-PARTICLE PACKINGS; DENSITY; SPHERES;
D O I
10.1103/PhysRevE.108.064602
中图分类号
O35 [流体力学]; O53 [等离子体物理学];
学科分类号
070204 ; 080103 ; 080704 ;
摘要
The maximally random jammed (MRJ) state is the most random configuration of strictly jammed (mechanically rigid) nonoverlapping objects. MRJ packings are hyperuniform, meaning their long-wavelength density fluctuations are anomalously suppressed compared to typical disordered systems, i.e., their structure factors S(k) tend to zero as the wavenumber |k| tends to zero. Here, we show that generating high-quality strictly jammed states for space dimensions d=3,4, and 5 is of paramount importance in ensuring hyperuniformity and extracting precise values of the hyperuniformity exponent alpha>0 for MRJ states, defined by the power-law behavior of S(k)similar to|k|(alpha) in the limit |k|-> 0. Moreover, we show that for fixed d it is more difficult to ensure jamming as the particle number N increases, which results in packings that are nonhyperuniform. Free-volume theory arguments suggest that the ideal MRJ state does not contain rattlers, which act as defects in numerically generated packings. As d increases, we find that the fraction of rattlers decreases substantially. Our analysis of the largest truly jammed packings suggests that the ideal MRJ packings for all dimensions d >= 3 are hyperuniform with alpha=d-2, implying the packings become more hyperuniform as d increases. The differences in alpha between MRJ packings and recently proposed Manna-class random close packed (RCP) states, which were reported to have alpha=0.25 in d=3 and be nonhyperuniform (alpha=0) for d=4 and d=5, demonstrate the vivid distinctions between the large-scale structure of RCP and MRJ states in these dimensions. Our work clarifies the importance of the link between true jamming and hyperuniformity and motivates the development of an algorithm to produce rattler-free three-dimensional MRJ packings.
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页数:12
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