Tomography of Feshbach resonance states

被引:9
|
作者
Margulis, Baruch [1 ]
Horn, Karl P. [2 ]
Reich, Daniel M. [2 ]
Upadhyay, Meenu [3 ]
Kahn, Nitzan [1 ]
Christianen, Arthur [4 ,5 ]
van der Avoird, Ad [5 ]
Groenenboom, Gerrit C. [5 ]
Koch, Christiane P. [2 ]
Meuwly, Markus [3 ]
Narevicius, Edvardas [1 ,6 ]
机构
[1] Weizmann Inst Sci, Dept Chem & Biol Phys, IL-7610001 Rehovot, Israel
[2] Free Univ Berlin, Dahlem Ctr Complex Quantum Syst & Fachbereich Phys, Arnimallee 14, D-14195 Berlin, Germany
[3] Univ Basel, Dept Chem, Basel, Switzerland
[4] Max Planck Inst Quantum Opt, Hans Kopfermann Str 1, D-85748 Garching, Germany
[5] Radboud Univ Nijmegen, Inst Mol & Mat, Theoret Chem, Heyendaalseweg 135, NL-6525 AJ Nijmegen, Netherlands
[6] Tech Univ, Dept Phys, Dortmund, Germany
基金
欧洲研究理事会;
关键词
ULTRACOLD; MOLECULES; DYNAMICS;
D O I
10.1126/science.adf9888
中图分类号
O [数理科学和化学]; P [天文学、地球科学]; Q [生物科学]; N [自然科学总论];
学科分类号
07 ; 0710 ; 09 ;
摘要
Feshbach resonances are fundamental to interparticle interactions and become particularly important in cold collisions with atoms, ions, and molecules. In this work, we present the detection of Feshbach resonances in a benchmark system for strongly interacting and highly anisotropic collisions: molecular hydrogen ions colliding with noble gas atoms. The collisions are launched by cold Penning ionization, which exclusively populates Feshbach resonances that span both short- and long-range parts of the interaction potential. We resolved all final molecular channels in a tomographic manner using ion-electron coincidence detection. We demonstrate the nonstatistical nature of the final-state distribution. By performing quantum scattering calculations on ab initio potential energy surfaces, we show that the isolation of the Feshbach resonance pathways reveals their distinctive fingerprints in the collision outcome.
引用
收藏
页码:77 / 81
页数:5
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