共 3 条
Historical trend of ozone-depleting substances and hydrofluorocarbon concentrations during 2004-2020 derived from satellite observations and estimates for global emissions
被引:7
|作者:
Chen, Ao
[1
,2
]
Chen, Di
[1
]
Hu, Xiaoyi
[1
]
Harth, Christina M.
[3
]
Young, Dickon
[4
]
Muehle, Jens
[3
]
Krummel, Paul B.
[5
]
O'Doherty, Simon
[4
]
Weiss, Ray F.
[3
]
Prinn, Ronald G.
[6
]
Fang, Xuekun
[1
,6
]
机构:
[1] Zhejiang Univ, Coll Environm & Resource Sci, Hangzhou, Zhejiang, Peoples R China
[2] Stanford Univ, Dept Civil & Environm Engn, Stanford, CA 94305 USA
[3] Univ Calif San Diego, Scripps Inst Oceanog, La Jolla, CA 92093 USA
[4] Univ Bristol, Sch Chem, Bristol, Avon, England
[5] CSIRO Oceans & Atmosphere, Climate Sci Ctr, Aspendale, Vic, Australia
[6] MIT, Ctr Global Change Sci, 77 Massachusetts Ave, Cambridge, MA 02139 USA
基金:
加拿大自然科学与工程研究理事会;
美国国家航空航天局;
中国国家自然科学基金;
关键词:
Ozone -depleting substance;
Concentration;
Emission;
Satellite ACE-FTS;
Montreal protocol;
METHYL-CHLORIDE;
AGAGE OBSERVATIONS;
CAPE GRIM;
CARBON-TETRACHLORIDE;
UPPER TROPOSPHERE;
VALIDATION;
ATMOSPHERE;
TASMANIA;
PROJECTIONS;
CFC-12;
D O I:
10.1016/j.envpol.2022.120570
中图分类号:
X [环境科学、安全科学];
学科分类号:
08 ;
0830 ;
摘要:
Global concentrations (or mole fractions) and emissions of ozone-depleting substances (ODSs) and their hydrofluorocarbon (HFCs) substitutes that are controlled by the Montreal Protocol and its Amendments and adjustments (MP) are of great interest to both the scientific community and public. Previous studies on global concentrations and emissions have mostly relied on ground-based observations. Here, we assess the global concentrations and emissions of eight MP controlled substances and methyl chloride from ACE-FTS (Atmospheric Chemistry Experiment high-resolution infrared Fourier transform spectrometer) satellite observations: CFC-11 (CFCl3), CFC-12 (CF2Cl2), CCl4, HCFC-22 (CHClF2), HCFC-141b (C2H3Cl2F), HCFC-142b (C2H3ClF2), HFC-23 (CHF3), HFC-134a (C2H2F4), and CH3Cl. Results show that the ACE-FTS satellite observations can be used to derive the concentrations and emissions of these ODSs, HFCs, and CH3Cl, as they are consistent with those derived from the ground-based observations. Our findings imply that the changes in the concentrations and emissions of the ODSs and HFCs closely match the regulatory status of the MP, and satellite observations can be used to monitor the past and future progress of the MP.
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页数:10
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